Polymer-decorated bacteria for cascade catalysis

IF 42.8 1区 化学 Q1 CHEMISTRY, PHYSICAL Nature Catalysis Pub Date : 2024-12-20 DOI:10.1038/s41929-024-01273-7
Andrea Belluati, Nico Bruns
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Abstract

Polymer/whole-cell hybrid catalysts were created by synthesizing catalytically active polymers from the surface of Escherichia coli cells that recombinantly expressed enzymes. The surface-engineered bacteria allowed for orthogonal tandem catalysis, involving photo- or chemocatalytic steps by the polymers on the cells and biocatalytic steps by the enzymes within the cells.

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用于级联催化的聚合物修饰细菌
聚合物/全细胞杂化催化剂是利用重组表达酶的大肠杆菌细胞表面合成具有催化活性的聚合物制备的。表面工程细菌允许进行正交串联催化,包括细胞上聚合物的光催化或化学催化步骤和细胞内酶的生物催化步骤。
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来源期刊
Nature Catalysis
Nature Catalysis Chemical Engineering-Bioengineering
CiteScore
52.10
自引率
1.10%
发文量
140
期刊介绍: Nature Catalysis serves as a platform for researchers across chemistry and related fields, focusing on homogeneous catalysis, heterogeneous catalysis, and biocatalysts, encompassing both fundamental and applied studies. With a particular emphasis on advancing sustainable industries and processes, the journal provides comprehensive coverage of catalysis research, appealing to scientists, engineers, and researchers in academia and industry. Maintaining the high standards of the Nature brand, Nature Catalysis boasts a dedicated team of professional editors, rigorous peer-review processes, and swift publication times, ensuring editorial independence and quality. The journal publishes work spanning heterogeneous catalysis, homogeneous catalysis, and biocatalysis, covering areas such as catalytic synthesis, mechanisms, characterization, computational studies, nanoparticle catalysis, electrocatalysis, photocatalysis, environmental catalysis, asymmetric catalysis, and various forms of organocatalysis.
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