{"title":"Overlooked calendar issues of aqueous zinc metal batteries","authors":"Bao Zhang, Hong Jin Fan","doi":"10.1016/j.joule.2024.12.003","DOIUrl":null,"url":null,"abstract":"Although the zinc metal plating and stripping chemistry offers a high specific capacity, this process suffers from poor reversibility, a crucial factor for long-term energy storage. Most studies so far have been focusing on cyclic aging but overlooked the impact of calendar aging on zinc metal behavior. In this perspective, we highlight the nearly cycle-independent and time-linear calendar aging mode of zinc metal anodes due to the lack of a protective solid-electrolyte interphase (SEI). This calendar aging could be the dominant factor in battery degradation throughout the entire life cycle. We advocate for a more critical evaluation of the battery lifespan and suggest strategies to circumvent calendar aging.","PeriodicalId":343,"journal":{"name":"Joule","volume":"8 1","pages":""},"PeriodicalIF":38.6000,"publicationDate":"2024-12-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Joule","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1016/j.joule.2024.12.003","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
Although the zinc metal plating and stripping chemistry offers a high specific capacity, this process suffers from poor reversibility, a crucial factor for long-term energy storage. Most studies so far have been focusing on cyclic aging but overlooked the impact of calendar aging on zinc metal behavior. In this perspective, we highlight the nearly cycle-independent and time-linear calendar aging mode of zinc metal anodes due to the lack of a protective solid-electrolyte interphase (SEI). This calendar aging could be the dominant factor in battery degradation throughout the entire life cycle. We advocate for a more critical evaluation of the battery lifespan and suggest strategies to circumvent calendar aging.
期刊介绍：
Joule is a sister journal to Cell that focuses on research, analysis, and ideas related to sustainable energy. It aims to address the global challenge of the need for more sustainable energy solutions. Joule is a forward-looking journal that bridges disciplines and scales of energy research. It connects researchers and analysts working on scientific, technical, economic, policy, and social challenges related to sustainable energy. The journal covers a wide range of energy research, from fundamental laboratory studies on energy conversion and storage to global-level analysis. Joule aims to highlight and amplify the implications, challenges, and opportunities of novel energy research for different groups in the field.
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