Andrew C Candia, Georg Bollen, Suvan Campbell, Ana Henriques, Alain Lapierre, Samuel Nash, Stefan Schwarz, Chandana Sumithrarachchi, Antonio C C Villari, Katharina A Domnanich
{"title":"Preparation of a <sup>73</sup>As source sample for application in an offline ion source.","authors":"Andrew C Candia, Georg Bollen, Suvan Campbell, Ana Henriques, Alain Lapierre, Samuel Nash, Stefan Schwarz, Chandana Sumithrarachchi, Antonio C C Villari, Katharina A Domnanich","doi":"10.1016/j.apradiso.2024.111642","DOIUrl":null,"url":null,"abstract":"<p><p>For the generation of beams with the offline ion source at the Facility for Rare Isotope Beams (FRIB), suitable source samples are required. Arsenic-73 is a frequently requested user beam due to its significance in nuclear structure studies and astrophysics. In this work, we outline the process of preparing a <sup>73</sup>As source sample, containing (5.76 ± 0.37)∗10<sup>14</sup> atoms of <sup>73</sup>As, which was successfully used to generate a <sup>73</sup>As beam for a multi-day user experiment. Silver arsenate was chosen as the chemical form, due to its favorable volatility within the designated operating temperature range. We refined the precipitation method using stable arsenic prior to its application with the <sup>73</sup>As sample, resulting in precipitation yields of (99.4 ± 4.5)%.</p>","PeriodicalId":8096,"journal":{"name":"Applied Radiation and Isotopes","volume":"217 ","pages":"111642"},"PeriodicalIF":1.6000,"publicationDate":"2025-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Applied Radiation and Isotopes","FirstCategoryId":"5","ListUrlMain":"https://doi.org/10.1016/j.apradiso.2024.111642","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2024/12/16 0:00:00","PubModel":"Epub","JCR":"Q3","JCRName":"CHEMISTRY, INORGANIC & NUCLEAR","Score":null,"Total":0}
引用次数: 0
Abstract
For the generation of beams with the offline ion source at the Facility for Rare Isotope Beams (FRIB), suitable source samples are required. Arsenic-73 is a frequently requested user beam due to its significance in nuclear structure studies and astrophysics. In this work, we outline the process of preparing a 73As source sample, containing (5.76 ± 0.37)∗1014 atoms of 73As, which was successfully used to generate a 73As beam for a multi-day user experiment. Silver arsenate was chosen as the chemical form, due to its favorable volatility within the designated operating temperature range. We refined the precipitation method using stable arsenic prior to its application with the 73As sample, resulting in precipitation yields of (99.4 ± 4.5)%.
期刊介绍:
Applied Radiation and Isotopes provides a high quality medium for the publication of substantial, original and scientific and technological papers on the development and peaceful application of nuclear, radiation and radionuclide techniques in chemistry, physics, biochemistry, biology, medicine, security, engineering and in the earth, planetary and environmental sciences, all including dosimetry. Nuclear techniques are defined in the broadest sense and both experimental and theoretical papers are welcome. They include the development and use of α- and β-particles, X-rays and γ-rays, neutrons and other nuclear particles and radiations from all sources, including radionuclides, synchrotron sources, cyclotrons and reactors and from the natural environment.
The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria.
Papers dealing with radiation processing, i.e., where radiation is used to bring about a biological, chemical or physical change in a material, should be directed to our sister journal Radiation Physics and Chemistry.