Surface Microstructure Enhanced Cryogenic Infrared Light Emitting Diodes for Semiconductor Broadband Upconversion.

IF 4.4 3区 材料科学 Q2 CHEMISTRY, MULTIDISCIPLINARY Nanomaterials Pub Date : 2024-12-19 DOI:10.3390/nano14242039
Peng Bai, Hanbin Wang, Rongrong Lv, Yi Wang, Yinqiao Li, Shangjie Han, Jiaxuan Cai, Ning Yang, Weidong Chu, Yan Xie, Meng Chen, Yingxin Wang, Ziran Zhao
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Abstract

Broadband upconversion has various applications in solar photovoltaic, infrared and terahertz detection imaging, and biomedicine. The low efficiency of the light-emitting diodes (LEDs) limits the broadband upconversion performance. In this paper, we propose to use surface microstructures to enhance the electroluminescence efficiency (ELE) of LEDs. Systematical investigations on the cryogenic-temperature performances of microstructure-coupled LEDs, including electroluminescence efficiency, luminescence spectrum, and recombination rate, have been carried out by elaborating their enhancement mechanism and light emitting characteristics both experimentally and theoretically. We have revealed that the reason for the nearly 35% ELE enhancement of the optimized structure under cryogenic temperature and weak injection current is the efficient carrier injection efficiency and the high recombination rate in the active region. We also compare studies of the surface luminescence uniformity of the optimized LED with that of the unoptimized device. This work gives a precise description, and explanation of the performance of the optimized microstructure coupled LED at low temperatures, providing important guidance and inspiration for the optimization of broadband upconverter in the cryogenic temperature region.

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用于半导体宽带上转换的表面微结构增强低温红外发光二极管。
宽带上变频在太阳能光伏、红外和太赫兹探测成像、生物医学等领域有着广泛的应用。发光二极管(led)的低效率限制了宽带上转换性能。本文提出利用表面微结构来提高led的电致发光效率(ELE)。系统研究了微结构耦合led的低温性能,包括电致发光效率、发光光谱和复合率,从实验和理论两方面阐述了微结构耦合led的增强机理和发光特性。结果表明,在低温弱注入电流条件下,优化结构的ELE增强近35%的原因是高效的载流子注入效率和活性区高的复合率。我们还比较了优化后的LED与未优化器件的表面发光均匀性。本工作对优化后的微结构耦合LED在低温下的性能进行了精确的描述和解释,为低温区宽带上变频器的优化提供了重要的指导和启示。
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来源期刊
Nanomaterials
Nanomaterials NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
8.50
自引率
9.40%
发文量
3841
审稿时长
14.22 days
期刊介绍: Nanomaterials (ISSN 2076-4991) is an international and interdisciplinary scholarly open access journal. It publishes reviews, regular research papers, communications, and short notes that are relevant to any field of study that involves nanomaterials, with respect to their science and application. Thus, theoretical and experimental articles will be accepted, along with articles that deal with the synthesis and use of nanomaterials. Articles that synthesize information from multiple fields, and which place discoveries within a broader context, will be preferred. There is no restriction on the length of the papers. Our aim is to encourage scientists to publish their experimental and theoretical research in as much detail as possible. Full experimental or methodical details, or both, must be provided for research articles. Computed data or files regarding the full details of the experimental procedure, if unable to be published in a normal way, can be deposited as supplementary material. Nanomaterials is dedicated to a high scientific standard. All manuscripts undergo a rigorous reviewing process and decisions are based on the recommendations of independent reviewers.
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