Albedo factors at 661.62 keV for several lanthanide compounds

IF 2.8 3区 物理与天体物理 Q3 CHEMISTRY, PHYSICAL Radiation Physics and Chemistry Pub Date : 2024-12-28 DOI:10.1016/j.radphyschem.2024.112492
Demet Yılmaz, Abdul Fatah Pathman, Sedanur Kalecik, Yakup Kurucu, Tuba Ö. Özer
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Abstract

Lanthanides, a group of rare earth elements, have attracted considerable attention due to their unique properties and valuable applications. In this study, the albedo parameters of three distinct groups of lanthanide compounds (Cerium, Gadolinium, and Samarium) were investigated using 661.62 keV gamma radiation emitted from a137Cs radioactive source and a high purity germanium detector in backscattering geometry. Additionally, the mass attenuation coefficients of lanthanide compounds were examined in absorption geometry. It was found that Cerium III fluoride, Gadolinium III sulfate, and Samarium III sulfate exhibit the highest albedo numbers among the lanthanide compounds. Furthermore, an exponential relationship between albedo values and mass attenuation coefficients was observed. This study concludes that molecular groups attached to the same atom can influence the photon scattering properties.
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几种镧系化合物的反照率因子为661.62 keV
镧系元素是一类稀土元素,由于其独特的性质和有价值的应用而受到广泛关注。在本研究中,利用a137Cs放射源发射的661.62 keV伽马射线和高纯度锗探测器,研究了三种不同类型的镧系化合物(铈、钆和钐)的反照率参数。此外,从吸收几何角度考察了镧系化合物的质量衰减系数。发现氟化铈、硫酸钆和硫酸钐的反照率在镧系化合物中最高。此外,反照率值与质量衰减系数呈指数关系。本研究认为,与同一原子相连的分子基团会影响光子的散射特性。
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来源期刊
Radiation Physics and Chemistry
Radiation Physics and Chemistry 化学-核科学技术
CiteScore
5.60
自引率
17.20%
发文量
574
审稿时长
12 weeks
期刊介绍: Radiation Physics and Chemistry is a multidisciplinary journal that provides a medium for publication of substantial and original papers, reviews, and short communications which focus on research and developments involving ionizing radiation in radiation physics, radiation chemistry and radiation processing. The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria. This could include papers that are very similar to previous publications, only with changed target substrates, employed materials, analyzed sites and experimental methods, report results without presenting new insights and/or hypothesis testing, or do not focus on the radiation effects.
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