Enhancing Water Electrolysis through Interfacial Design of Nickel Foam

IF 3.9 2区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY Langmuir Pub Date : 2025-01-10 DOI:10.1021/acs.langmuir.4c04714
Lingling Sun, Yi Zeng, Jitao Li, Haoqi Wang, Qingsong Hua, Shun Lu
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Abstract

Water electrolysis recognizes nickel foam (NF) as an effective current collector due to its excellent conductivity. However, recent studies highlighted NF’s effect on the efficacy of various electrocatalytic reactions, primarily due to the presence of electroactive chemical species at its interface. In contrast, numerous reports suggested that NF has a negligible impact on overall electrocatalytic activity. When evaluated against other current collectors, NF-supported catalysts demonstrate better electrochemical activity, predominantly due to NF’s interfacial design. This study presents an electrochemically relevant NF with a flexible interfacial design, supported by case studies and insights into promising future directions. This Perspective reveals the advantages, challenges, and overall applicability of NF’s interfacial design with the context of electrocatalytic water splitting in mind.

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泡沫镍界面设计提高水的电解性能
由于泡沫镍具有优异的导电性,因此在水电解过程中被认为是一种有效的集流剂。然而,最近的研究强调了NF对各种电催化反应效果的影响,主要是由于其界面上存在电活性化学物质。相反,许多报告表明,NF对整体电催化活性的影响可以忽略不计。当与其他电流收集器进行比较时,NF支持的催化剂表现出更好的电化学活性,这主要是由于NF的界面设计。本研究提出了一个与电化学相关的NF,具有灵活的界面设计,并通过案例研究和对未来发展方向的洞察来支持。本文从电催化水分解的角度,揭示了NF界面设计的优势、挑战和整体适用性。
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来源期刊
Langmuir
Langmuir 化学-材料科学:综合
CiteScore
6.50
自引率
10.30%
发文量
1464
审稿时长
2.1 months
期刊介绍: Langmuir is an interdisciplinary journal publishing articles in the following subject categories: Colloids: surfactants and self-assembly, dispersions, emulsions, foams Interfaces: adsorption, reactions, films, forces Biological Interfaces: biocolloids, biomolecular and biomimetic materials Materials: nano- and mesostructured materials, polymers, gels, liquid crystals Electrochemistry: interfacial charge transfer, charge transport, electrocatalysis, electrokinetic phenomena, bioelectrochemistry Devices and Applications: sensors, fluidics, patterning, catalysis, photonic crystals However, when high-impact, original work is submitted that does not fit within the above categories, decisions to accept or decline such papers will be based on one criteria: What Would Irving Do? Langmuir ranks #2 in citations out of 136 journals in the category of Physical Chemistry with 113,157 total citations. The journal received an Impact Factor of 4.384*. This journal is also indexed in the categories of Materials Science (ranked #1) and Multidisciplinary Chemistry (ranked #5).
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