Emission of electrons and photons and formation of cascade ions during the decay of 125I radionuclide

IF 2.3 3区 物理与天体物理 Q2 OPTICS Journal of Quantitative Spectroscopy & Radiative Transfer Pub Date : 2025-01-09 DOI:10.1016/j.jqsrt.2025.109348
A.P. Chaynikov, A.G. Kochur, A.I. Dudenko
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Abstract

Emission of electrons and photons during the cascade decay of inner-shell vacancies created after the decay of unstable 125I radionuclide is simulated by construction and analysis of the cascade decay trees in isolated-ion approximation. The yields of final cascade ions, the number of emitted electrons and photons, and their spectra, are calculated. During one transformation of 125I, the total energy emitted to the environment is 61.7 keV, of which 43.3 keV is emitted by photons, mostly high-energy KL photons produced at the first step of the decays of the 1s vacancies. If 125I is used as an agent for Auger therapy of cancer, only the energy absorbed by the tumor tissues in the nearest vicinity of the emitter is important. This energy is 18.6 keV, most of which is provided by cascade-produced electrons. The contribution of low-energy photons and cascade-produced ions to local energy deposition are 0.15 keV and 0.7 keV, respectively. Additional monopole ejection of electrons (shake off) during the cascades progression, and upon the internal conversion of 125Te* nuclide produced by the electron capture decay of 125I, is shown to affect little the final ions charges and emitted energies.
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125I 放射性核素衰变过程中电子和光子的发射以及级联离子的形成
通过构建和分析孤立离子近似的级联衰变树,模拟了不稳定的125I核素衰变后产生的内壳空位级联衰变过程中电子和光子的发射。计算了最终级联离子的产率、发射的电子和光子的数量以及它们的光谱。在125I的一次转化过程中,向环境发射的总能量为61.7 keV,其中43.3 keV是由光子发射的,主要是1s空位衰变第一步产生的高能KL光子。如果125I被用作癌症的俄歇治疗剂,那么只有靠近发射器的肿瘤组织所吸收的能量才是重要的。该能量为18.6 keV,其中大部分由级联产生的电子提供。低能光子和级联离子对局部能量沉积的贡献分别为0.15 keV和0.7 keV。在级联过程中,以及在125I的电子捕获衰变产生的125Te*核素的内部转换过程中,显示出额外的单极子喷射电子(摆脱)对最终离子电荷和发射能量的影响很小。
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来源期刊
CiteScore
5.30
自引率
21.70%
发文量
273
审稿时长
58 days
期刊介绍: Papers with the following subject areas are suitable for publication in the Journal of Quantitative Spectroscopy and Radiative Transfer: - Theoretical and experimental aspects of the spectra of atoms, molecules, ions, and plasmas. - Spectral lineshape studies including models and computational algorithms. - Atmospheric spectroscopy. - Theoretical and experimental aspects of light scattering. - Application of light scattering in particle characterization and remote sensing. - Application of light scattering in biological sciences and medicine. - Radiative transfer in absorbing, emitting, and scattering media. - Radiative transfer in stochastic media.
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