A cryogenic CO2 capture system coupled with boil-off gas re-liquefaction for LNG carriers

IF 9 1区 工程技术 Q1 ENGINEERING, CHEMICAL Separation and Purification Technology Pub Date : 2025-01-23 DOI:10.1016/j.seppur.2025.131783
Gequn Shu, Borui Liu, Hua Tian, Ligeng Li, Rui Sun, Xuan Wang
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Abstract

With the rising global demand for liquefied natural gas (LNG) in various fields, the need for LNG carriers has increased, which causes elevated CO2 emission. Thus, CO2 capture technology to achieve carbon neutrality on large LNG carriers has become a research concern. Besides, boil-off gas (BOG) is constantly generated which is due to the unavoidable heat leaks during the voyage resulting in the vaporization of several LNG. Therefore, a novel cryogenic on-board carbon capture (COCC) system making full use of LNG cold energy coupled with a BOG re-liquefaction (COCC-RL) system is firstly proposed, and the full operation conditions are considered. In this integrated system, superior thermal matching allows for CO2 capture in the exhaust, natural gas fuel vaporization and BOG re-liquefaction. It is astounding that the small capacity capture system could also produce a more competitive annual total profit (ATP) (4.13 × 104 $/ton) at a higher CO2 capture rate (56.69 %) compared to a high main load as design point. Therefore, a hitherto unexploited solution avenue has emerged, presenting a novel direction for designing a cryogenic on-board carbon capture system coupled with BOG re-liquefaction at variable engine loads and shows the potential of cryogenic CO2 capture technology in the shipping industry.
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LNG运输船的低温CO2捕集系统与蒸发气体再液化相结合
随着全球各个领域对液化天然气(LNG)需求的增加,LNG运输船的需求也随之增加,这导致了二氧化碳排放量的增加。因此,在大型液化天然气运输船上实现碳中和的二氧化碳捕集技术已成为一个研究热点。此外,由于航行中不可避免的热泄漏导致一些液化天然气汽化,不断产生汽化气(BOG)。为此,首次提出了一种充分利用LNG冷能并结合BOG再液化的新型低温车载碳捕集(COCC)系统,并考虑了该系统的全工况。在这个集成系统中,卓越的热匹配允许废气中的二氧化碳捕获,天然气燃料蒸发和BOG再液化。令人震惊的是,与高主负荷设计点相比,小容量捕集系统也可以在更高的二氧化碳捕集率(56.69 %)下产生更具竞争力的年总利润(ATP)(4.13 × 104美元/吨)。因此,一个迄今为止尚未开发的解决方案已经出现,为设计一个低温车载碳捕集系统以及在可变发动机负载下的BOG再液化提供了一个新的方向,并显示了低温二氧化碳捕集技术在航运业的潜力。
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来源期刊
Separation and Purification Technology
Separation and Purification Technology 工程技术-工程:化工
CiteScore
14.00
自引率
12.80%
发文量
2347
审稿时长
43 days
期刊介绍: Separation and Purification Technology is a premier journal committed to sharing innovative methods for separation and purification in chemical and environmental engineering, encompassing both homogeneous solutions and heterogeneous mixtures. Our scope includes the separation and/or purification of liquids, vapors, and gases, as well as carbon capture and separation techniques. However, it's important to note that methods solely intended for analytical purposes are not within the scope of the journal. Additionally, disciplines such as soil science, polymer science, and metallurgy fall outside the purview of Separation and Purification Technology. Join us in advancing the field of separation and purification methods for sustainable solutions in chemical and environmental engineering.
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