Aijia Zhang , Yong Wang , Yueyue Ma , Qingzheng Jia , Ling Li , Youwei Zhao , Yucang Zhang , Wenming Zhang
{"title":"Multi-layer fabric assembly ultra-high sensitivity dynamic anti-crosstalk sensing interactive interface based on secondary-enhanced microstructure for multi-task detection","authors":"Aijia Zhang , Yong Wang , Yueyue Ma , Qingzheng Jia , Ling Li , Youwei Zhao , Yucang Zhang , Wenming Zhang","doi":"10.1016/j.cej.2025.159938","DOIUrl":null,"url":null,"abstract":"<div><div>Wearable electronic devices are important interfaces for human motion detection and human–computer interaction. However, the current sensing equipment has low sensitivity and poor crosstalk prevention capability, which cannot meet the demand. Herein, we propose a secondary enhanced electrode fabrication strategy for the preparation of multifunctional sensors. The sensor consists of a top electrode CC@NiAl-LDH with a secondary enhancement structure, the photo-reticulated strain localization films (prslPDMS) as the separator layer, and a bottom electrode silver nanowire layer. The synergistic effect of the prslPDMS and the top electrode sensing layer improves the anti-crosstalk ability and sensitivity of this sensor. Among them, CC@NiAl-LDH is not only used as a material for piezoresistive sensors, but also selected as a key component of TENG due to its excellent triboelectric properties. The structural advantages of prslPDMS and CC@NiAl-LDH as the sensing layer are verified by finite element simulation analysis. The designed sensor boasts an ultra-wide detection range (0–2000 kPa), ultra-high sensitivity (3.9 × 10<sup>9</sup> kPa<sup>−1</sup>), and rapid response and recovery times (25/30 ms). In addition, through the integration of machine learning algorithms, a multi-signal recognition system compatible with a variety of signal acquisition and analysis functions was designed, realizing multi-signal, multi-dimensional and high-precision recognition of sign language gestures, with an accuracy rate of more than 93 % for 15 gestures. This represents a significant milestone in the development of human–computer interaction. In addation direction of LDHs is also oriented towards application of NiAl-LDH materials in the field of triboelectric nanogenerators. Preliminary research showed that it has the ability to convert into electrical energy, providing new possibilities for self-powered systems in future wearable devices.</div></div>","PeriodicalId":270,"journal":{"name":"Chemical Engineering Journal","volume":"506 ","pages":"Article 159938"},"PeriodicalIF":13.3000,"publicationDate":"2025-01-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Chemical Engineering Journal","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1385894725007375","RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
引用次数: 0
Abstract
Wearable electronic devices are important interfaces for human motion detection and human–computer interaction. However, the current sensing equipment has low sensitivity and poor crosstalk prevention capability, which cannot meet the demand. Herein, we propose a secondary enhanced electrode fabrication strategy for the preparation of multifunctional sensors. The sensor consists of a top electrode CC@NiAl-LDH with a secondary enhancement structure, the photo-reticulated strain localization films (prslPDMS) as the separator layer, and a bottom electrode silver nanowire layer. The synergistic effect of the prslPDMS and the top electrode sensing layer improves the anti-crosstalk ability and sensitivity of this sensor. Among them, CC@NiAl-LDH is not only used as a material for piezoresistive sensors, but also selected as a key component of TENG due to its excellent triboelectric properties. The structural advantages of prslPDMS and CC@NiAl-LDH as the sensing layer are verified by finite element simulation analysis. The designed sensor boasts an ultra-wide detection range (0–2000 kPa), ultra-high sensitivity (3.9 × 109 kPa−1), and rapid response and recovery times (25/30 ms). In addition, through the integration of machine learning algorithms, a multi-signal recognition system compatible with a variety of signal acquisition and analysis functions was designed, realizing multi-signal, multi-dimensional and high-precision recognition of sign language gestures, with an accuracy rate of more than 93 % for 15 gestures. This represents a significant milestone in the development of human–computer interaction. In addation direction of LDHs is also oriented towards application of NiAl-LDH materials in the field of triboelectric nanogenerators. Preliminary research showed that it has the ability to convert into electrical energy, providing new possibilities for self-powered systems in future wearable devices.
期刊介绍:
The Chemical Engineering Journal is an international research journal that invites contributions of original and novel fundamental research. It aims to provide an international platform for presenting original fundamental research, interpretative reviews, and discussions on new developments in chemical engineering. The journal welcomes papers that describe novel theory and its practical application, as well as those that demonstrate the transfer of techniques from other disciplines. It also welcomes reports on carefully conducted experimental work that is soundly interpreted. The main focus of the journal is on original and rigorous research results that have broad significance. The Catalysis section within the Chemical Engineering Journal focuses specifically on Experimental and Theoretical studies in the fields of heterogeneous catalysis, molecular catalysis, and biocatalysis. These studies have industrial impact on various sectors such as chemicals, energy, materials, foods, healthcare, and environmental protection.