Aloof Electron Probing of In-Plane Surface Photovoltaic Charge Distributions on GaAs Surfaces

IF 6.5 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Photonics Pub Date : 2025-01-27 DOI:10.1021/acsphotonics.4c01997
Zilin Chen, Wayne Cheng-Wei Huang, Herman Batelaan
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Abstract

The motion of free electrons moving parallel and above a semiconductor surface can be influenced by shining a laser light onto the surface. Here we report strong deflection of aloof electrons by an undoped GaAs surface illuminated with a 633 nm laser. The deflecting electric field from the surface photovoltaic charges extends 100 μm into the vacuum. As surface photovoltage (SPV) is sensitive to the electronic states of the GaAs surface, the aloof electron beam serves as a probe for SPV charge dynamics on the mesoscopic length scale. The observed in-plane SPV charge distribution persists beyond 1 second after the laser beam is blocked. Our work suggests the possibility of writing designed 2D charge patterns on semiconductor surfaces with a scanning laser beam, providing unusual flexibility for electron beam manipulation.

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平行于半导体表面运动的自由电子的运动可以受到照射到表面的激光的影响。在此,我们报告了在 633 纳米激光照射下,未掺杂砷化镓表面对自由电子的强烈偏转。来自表面光电荷的偏转电场向真空中延伸了 100 μm。由于表面光电电压(SPV)对砷化镓表面的电子状态非常敏感,因此冷电子束可作为介观长度尺度上 SPV 电荷动态的探针。观察到的平面内 SPV 电荷分布在激光束被阻挡后持续了 1 秒钟以上。我们的工作表明,利用扫描激光束可以在半导体表面写入设计好的二维电荷图案,为电子束操纵提供了非同寻常的灵活性。
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来源期刊
ACS Photonics
ACS Photonics NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
11.90
自引率
5.70%
发文量
438
审稿时长
2.3 months
期刊介绍: Published as soon as accepted and summarized in monthly issues, ACS Photonics will publish Research Articles, Letters, Perspectives, and Reviews, to encompass the full scope of published research in this field.
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