Migrating characteristics of pollutants from landfill leachate in cold regions and impact on hydrothermal conditions

IF 10 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Journal of Cleaner Production Pub Date : 2025-02-15 Epub Date: 2025-01-27 DOI:10.1016/j.jclepro.2025.144882
Han Jia , Shujuan Zhang , Zhizhong Sun , Yapeng Wang , Ruiqiang Bai
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Abstract

Economic development, unique tourism resources, and lifestyle changes of herdsmen in the Qinghai-Tibet Plateau (QTP) have resulted in an increasing waste disposal problem and most of the domestic waste was dumped into garbage pits for open burning and simple landfills in the rural and pastoral areas of Tibet. However, knowledge about heat transfer, water, and pollutant transport from landfill leachate in cold regions is currently limited. A series of migration tests were carried out under freeze-thaw cycles (FTCs), analyzing the distribution of temperature, water, and pollutants from the landfill leachate (main components include ammonia nitrogen (AN), chemical oxygen demand (COD), and cadmium (Cd)). The results show that the distribution of temperature, water, and pollutants in frozen soil is closely related to FTCs, water migration, boundary temperature, and the polluted degree of soil. The response degree to the top temperature is largest, secondary, and smallest for the unpolluted, polluted, and polluting soil, respectively. In the polluting soil, with the increasing FTCs, the content of AN, Cd, and COD also increases, and the water content mainly increases in the first 5 cycles. AN and COD are mainly adsorbed in the shallow layer, and Cd is enriched in the bottom where the temperature is close to the initial freezing one. The higher the boundary temperature, the greater the adsorption capacity for AN and COD, and the smaller the enriched content of Cd in the measured depth. AN and Cd are more easily adsorbed or removed than COD.
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寒冷地区垃圾填埋场沥滤液污染物的迁移特征及其对热液条件的影响
青藏高原经济的发展、独特的旅游资源和牧民生活方式的改变,导致生活垃圾处理问题日益严重,西藏农牧区的生活垃圾大多被倾倒到垃圾坑中露天焚烧和简单填埋。然而,关于寒冷地区垃圾填埋场渗滤液的传热、水和污染物运输的知识目前有限。在冻融循环(FTCs)条件下进行了一系列迁移试验,分析了填埋场渗滤液的温度、水和污染物(主要成分为氨氮(AN)、化学需氧量(COD)和镉(Cd))的分布。结果表明:冻土中温度、水分和污染物的分布与FTCs、水分迁移、边界温度和土壤污染程度密切相关。未污染土壤、污染土壤和污染土壤对最高温度的响应程度最大、次之、最小。在污染土壤中,随着FTCs的增加,AN、Cd和COD的含量也增加,含水量主要在前5个循环中增加。AN和COD主要吸附在浅层,Cd富集在接近初始冻结温度的底部。边界温度越高,对AN和COD的吸附能力越大,Cd在测量深度的富集含量越小。AN和Cd比COD更容易吸附或去除。
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来源期刊
Journal of Cleaner Production
Journal of Cleaner Production 环境科学-工程:环境
CiteScore
20.40
自引率
9.00%
发文量
4720
审稿时长
111 days
期刊介绍: The Journal of Cleaner Production is an international, transdisciplinary journal that addresses and discusses theoretical and practical Cleaner Production, Environmental, and Sustainability issues. It aims to help societies become more sustainable by focusing on the concept of 'Cleaner Production', which aims at preventing waste production and increasing efficiencies in energy, water, resources, and human capital use. The journal serves as a platform for corporations, governments, education institutions, regions, and societies to engage in discussions and research related to Cleaner Production, environmental, and sustainability practices.
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