Room-temperature continuous-wave pumped exciton polariton condensation in a perovskite microcavity

IF 12.5 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Science Advances Pub Date : 2025-01-29 DOI:10.1126/sciadv.adr1652
Jiepeng Song, Sanjib Ghosh, Xinyi Deng, Chun Li, Qiuyu Shang, Xinfeng Liu, Yubin Wang, Xiaoyue Gao, Wenkai Yang, Xianjin Wang, Qing Zhao, Kebin Shi, Peng Gao, Guichuan Xing, Qihua Xiong, Qing Zhang
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Abstract

Microcavity exciton polaritons (polaritons) as part-light part-matter quasiparticles garner considerable attention for Bose-Einstein condensation at elevated temperatures. Recently, halide perovskites have emerged as promising room-temperature polaritonic platforms because of their large exciton binding energies and superior optical properties. However, currently, inducing room-temperature nonequilibrium polariton condensation in perovskite microcavities requires optical pulsed excitations with high excitation densities. Here, we demonstrate continuous-wave optically pumped polariton condensation with an exceptionally low threshold of ~0.53 W cm−2 and a narrow linewidth of ~0.5 meV. Polariton condensation is unambiguously demonstrated by characterizing the nonlinear behavior and coherence properties. We also unveil the trapping potential landscape strategy to facilitate polariton relaxation and accumulation. Our findings lay the foundation for the next-generation energy-efficient polaritonic devices operating at room temperature.

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钙钛矿微腔中室温连续波泵浦激子极化子凝聚。
微腔激子极化子作为半光半物质准粒子在高温下的玻色-爱因斯坦凝聚中引起了相当大的关注。近年来,卤化物钙钛矿因其巨大的激子结合能和优越的光学特性而成为有前途的室温极化平台。然而,目前,在钙钛矿微腔中诱导室温非平衡极化子凝聚需要高激发密度的光脉冲激发。在这里,我们展示了连续波光泵浦极化子凝聚,具有非常低的阈值~0.53 W cm-2和~0.5 meV的窄线宽。极化子凝聚通过表征非线性行为和相干特性得到了明确的证明。我们还揭示了捕获潜在景观策略,以促进极化子的松弛和积累。我们的研究结果为在室温下工作的下一代节能极化器件奠定了基础。
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来源期刊
Science Advances
Science Advances 综合性期刊-综合性期刊
CiteScore
21.40
自引率
1.50%
发文量
1937
审稿时长
29 weeks
期刊介绍: Science Advances, an open-access journal by AAAS, publishes impactful research in diverse scientific areas. It aims for fair, fast, and expert peer review, providing freely accessible research to readers. Led by distinguished scientists, the journal supports AAAS's mission by extending Science magazine's capacity to identify and promote significant advances. Evolving digital publishing technologies play a crucial role in advancing AAAS's global mission for science communication and benefitting humankind.
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