Room-temperature continuous-wave pumped exciton polariton condensation in a perovskite microcavity

IF 11.7 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Science Advances Pub Date : 2025-01-29 DOI:10.1126/sciadv.adr1652
Jiepeng Song, Sanjib Ghosh, Xinyi Deng, Chun Li, Qiuyu Shang, Xinfeng Liu, Yubin Wang, Xiaoyue Gao, Wenkai Yang, Xianjin Wang, Qing Zhao, Kebin Shi, Peng Gao, Guichuan Xing, Qihua Xiong, Qing Zhang
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Abstract

Microcavity exciton polaritons (polaritons) as part-light part-matter quasiparticles garner considerable attention for Bose-Einstein condensation at elevated temperatures. Recently, halide perovskites have emerged as promising room-temperature polaritonic platforms because of their large exciton binding energies and superior optical properties. However, currently, inducing room-temperature nonequilibrium polariton condensation in perovskite microcavities requires optical pulsed excitations with high excitation densities. Here, we demonstrate continuous-wave optically pumped polariton condensation with an exceptionally low threshold of ~0.53 W cm−2 and a narrow linewidth of ~0.5 meV. Polariton condensation is unambiguously demonstrated by characterizing the nonlinear behavior and coherence properties. We also unveil the trapping potential landscape strategy to facilitate polariton relaxation and accumulation. Our findings lay the foundation for the next-generation energy-efficient polaritonic devices operating at room temperature.

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来源期刊
Science Advances
Science Advances 综合性期刊-综合性期刊
CiteScore
21.40
自引率
1.50%
发文量
1937
审稿时长
29 weeks
期刊介绍: Science Advances, an open-access journal by AAAS, publishes impactful research in diverse scientific areas. It aims for fair, fast, and expert peer review, providing freely accessible research to readers. Led by distinguished scientists, the journal supports AAAS's mission by extending Science magazine's capacity to identify and promote significant advances. Evolving digital publishing technologies play a crucial role in advancing AAAS's global mission for science communication and benefitting humankind.
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