{"title":"Determination of self-attenuation correction factors for 3′′×3′′ NaI(Tl) detector by using Monte Carlo Code FLUKA","authors":"Hakan Çetinkaya","doi":"10.1016/j.radphyschem.2025.112560","DOIUrl":null,"url":null,"abstract":"<div><div>NaI(Tl) gamma spectroscopy systems are widely used to determine the radioactivity level of the environmental samples. It is important to calculate the correct activity of environmental samples with respect to the calibration source. An activity correction is required when the density or absorption coefficient of the calibration source and the environmental sample is different; this is called the self-attenuation correction factor. In this study, the <span><math><mrow><msup><mrow><mn>3</mn></mrow><mrow><mo>′</mo><mo>′</mo></mrow></msup><mo>×</mo><msup><mrow><mn>3</mn></mrow><mrow><mo>′</mo><mo>′</mo></mrow></msup></mrow></math></span> NaI(Tl) gamma spectroscopy system in our laboratory was modeled using the Monte Carlo code FLUKA. Simulation results were validated by comparing the experimental and simulation FWHM results both for disk sources alone and disk sources placed above the 1 L Marinelli beakers. Self-attenuation correction factors were calculated for 0.5 and 1 L Marinelli beakers in the <span><math><mrow><mn>238</mn><mo>.</mo><mn>6</mn><mtext>-</mtext><mn>2614</mn></mrow></math></span> keV energy range using the FLUKA code. The materials in Marinelli beakers are assumed to be air, water and <span><math><msub><mrow><mi>SiO</mi></mrow><mrow><mn>2</mn></mrow></msub></math></span> in FLUKA simulations, the densities of these materials range from 0 to 2.8 <span><math><mrow><mi>g</mi><mo>/</mo><msup><mrow><mi>cm</mi></mrow><mrow><mn>3</mn></mrow></msup></mrow></math></span>. Additionally, energy and material density dependent coefficients of the analytical self-attenuation correction factor equation for 0.5 and 1 L Marinelli beakers were also derived using the FLUKA results.</div></div>","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"230 ","pages":"Article 112560"},"PeriodicalIF":2.8000,"publicationDate":"2025-01-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Radiation Physics and Chemistry","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0969806X25000520","RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
NaI(Tl) gamma spectroscopy systems are widely used to determine the radioactivity level of the environmental samples. It is important to calculate the correct activity of environmental samples with respect to the calibration source. An activity correction is required when the density or absorption coefficient of the calibration source and the environmental sample is different; this is called the self-attenuation correction factor. In this study, the NaI(Tl) gamma spectroscopy system in our laboratory was modeled using the Monte Carlo code FLUKA. Simulation results were validated by comparing the experimental and simulation FWHM results both for disk sources alone and disk sources placed above the 1 L Marinelli beakers. Self-attenuation correction factors were calculated for 0.5 and 1 L Marinelli beakers in the keV energy range using the FLUKA code. The materials in Marinelli beakers are assumed to be air, water and in FLUKA simulations, the densities of these materials range from 0 to 2.8 . Additionally, energy and material density dependent coefficients of the analytical self-attenuation correction factor equation for 0.5 and 1 L Marinelli beakers were also derived using the FLUKA results.
NaI(Tl)伽马能谱系统被广泛用于环境样品的放射性水平测定。计算环境样品相对于校准源的正确活度是很重要的。当校准源与环境样品的密度或吸收系数不同时,需要进行活度校正;这被称为自衰减校正因子。在本研究中,我们实验室的3“×3”NaI(Tl)伽马能谱系统使用蒙特卡罗代码FLUKA进行建模。通过比较单独的圆盘源和放置在1l Marinelli烧杯上方的圆盘源的实验结果和仿真结果,验证了仿真结果。使用FLUKA代码计算了能量范围为238.6-2614 keV的0.5 L和1 L Marinelli烧杯的自衰减校正因子。在FLUKA模拟中,马里内利烧杯中的材料被假设为空气、水和SiO2,这些材料的密度范围为0到2.8 g/cm3。此外,还利用FLUKA结果推导了0.5 L和1 L Marinelli烧杯解析自衰减校正因子方程的能量和材料密度依赖系数。
期刊介绍:
Radiation Physics and Chemistry is a multidisciplinary journal that provides a medium for publication of substantial and original papers, reviews, and short communications which focus on research and developments involving ionizing radiation in radiation physics, radiation chemistry and radiation processing.
The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria. This could include papers that are very similar to previous publications, only with changed target substrates, employed materials, analyzed sites and experimental methods, report results without presenting new insights and/or hypothesis testing, or do not focus on the radiation effects.