High-Resolution Dual-Energy X-ray Imaging Enabled by Transparent Thermally Activated Delayed Fluorescence (TADF) Scintillation Screen

IF 8.7 1区 化学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Materials Letters Pub Date : 2024-12-16 DOI:10.1021/acsmaterialslett.4c02203
Jian-Xin Wang, Tengyue He, Xin Zhu, Simil Thomas, Wenyi Shao, Osama Shekhah, Husam N. Alshareef, Osman M. Bakr, Mohamed Eddaoudi and Omar F. Mohammed*, 
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Abstract

Dual-energy X-ray imaging technology provides more detailed material-specific information by using a second X-ray spectrum. However, conventional dual-energy X-ray imaging typically necessitates two separate exposures to combine high- and low-energy projections. This process can result in image misalignment and increased radiation doses. Herein, a dual-energy X-ray imaging system using a two-layered scintillator was developed, featuring transparent pure organic thermally activated delayed fluorescence (TADF) materials as the low-energy absorption layer and LYSO as the high-energy absorption layer. Separating the energy bins on the detector side enables the simultaneous and sequential acquisition of low- and high-energy projections with a single X-ray exposure. This two-layered scintillator achieves a high imaging resolution of 23 lp/mm, surpassing most conventional single-layer scintillators. Additionally, the effectiveness of this dual-energy imaging system was demonstrated in a toolbox inspection, where complex objects inside were successfully imaged and differentiated, capturing all intricate details in a single X-ray exposure.

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透明热激活延迟荧光(TADF)闪烁屏实现高分辨率双能x射线成像
双能x射线成像技术通过使用第二个x射线光谱提供更详细的材料特定信息。然而,传统的双能x射线成像通常需要两次单独的曝光来结合高能量和低能投影。这一过程可能导致图像错位和辐射剂量增加。本文研制了以透明纯有机热激活延迟荧光(TADF)材料为低能吸收层,LYSO为高能吸收层的双层闪烁体双能x射线成像系统。在探测器侧分离能量仓,可以通过单个x射线曝光同时和顺序地获取低能和高能投影。这种双层闪烁体实现了23 lp/mm的高成像分辨率,超过了大多数传统的单层闪烁体。此外,这种双能成像系统的有效性在工具箱检查中得到了证明,其中复杂物体的内部成功成像和区分,在一次x射线曝光中捕获了所有复杂的细节。
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来源期刊
ACS Materials Letters
ACS Materials Letters MATERIALS SCIENCE, MULTIDISCIPLINARY-
CiteScore
14.60
自引率
3.50%
发文量
261
期刊介绍: ACS Materials Letters is a journal that publishes high-quality and urgent papers at the forefront of fundamental and applied research in the field of materials science. It aims to bridge the gap between materials and other disciplines such as chemistry, engineering, and biology. The journal encourages multidisciplinary and innovative research that addresses global challenges. Papers submitted to ACS Materials Letters should clearly demonstrate the need for rapid disclosure of key results. The journal is interested in various areas including the design, synthesis, characterization, and evaluation of emerging materials, understanding the relationships between structure, property, and performance, as well as developing materials for applications in energy, environment, biomedical, electronics, and catalysis. The journal has a 2-year impact factor of 11.4 and is dedicated to publishing transformative materials research with fast processing times. The editors and staff of ACS Materials Letters actively participate in major scientific conferences and engage closely with readers and authors. The journal also maintains an active presence on social media to provide authors with greater visibility.
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