Jose Eduardo Ubillus , Sahar Bakhshian , Hailun Ni , David DiCarlo , Tip Meckel
{"title":"Informing field-scale CO2storage simulations with sandbox experiments: The effect of small-scale heterogeneities","authors":"Jose Eduardo Ubillus , Sahar Bakhshian , Hailun Ni , David DiCarlo , Tip Meckel","doi":"10.1016/j.ijggc.2025.104318","DOIUrl":null,"url":null,"abstract":"<div><div>Small-scale heterogeneities can significantly affect the fate of the <span><math><mrow><mi>C</mi><msub><mrow><mi>O</mi></mrow><mrow><mn>2</mn></mrow></msub></mrow></math></span> plume and trapping during CO<span><math><mrow><msub><mrow></mrow><mrow><mn>2</mn></mrow></msub><mspace></mspace></mrow></math></span>migration. We conducted geologic carbon storage field-scale simulations to investigate the impact of small-scale heterogeneities on plume dynamics and trapping performance. Small-scale heterogeneities have been shown to increase the amount of trapped CO<span><math><mrow><msub><mrow></mrow><mrow><mn>2</mn></mrow></msub><mspace></mspace></mrow></math></span>during buoyancy-driven flow. The trapped <span><math><mrow><mi>C</mi><msub><mrow><mi>O</mi></mrow><mrow><mn>2</mn></mrow></msub></mrow></math></span> saturation is validated by previous sandbox experimental work during buoyancy-driven flow in realistic heterogeneous domains and is implemented through the critical CO<span><math><mrow><msub><mrow></mrow><mrow><mn>2</mn></mrow></msub><mspace></mspace></mrow></math></span>saturation parameter (i.e., the first non-zero value in the drainage CO<span><math><mrow><msub><mrow></mrow><mrow><mn>2</mn></mrow></msub><mspace></mspace></mrow></math></span>relative permeability curve). Depending on the type and degree of heterogeneity, various critical CO<span><math><mrow><msub><mrow></mrow><mrow><mn>2</mn></mrow></msub><mspace></mspace></mrow></math></span>saturation values are exhibited. Furthermore, we investigated the effect of small-scale heterogeneties when multiple capillary pressure models are employed. This study demonstrates that an increase in critical CO<span><math><mrow><msub><mrow></mrow><mrow><mn>2</mn></mrow></msub><mspace></mspace></mrow></math></span>saturation reduces the CO<span><math><mrow><msub><mrow></mrow><mrow><mn>2</mn></mrow></msub><mspace></mspace></mrow></math></span>plume size and lateral extent, accompanying an increase in residual trapping and a decrease in solubility trapping. Finally, we show that independent of the capillary pressure model used, an increase in critical saturation leads to similar CO<span><math><mrow><msub><mrow></mrow><mrow><mn>2</mn></mrow></msub><mspace></mspace></mrow></math></span>plume dynamics distribution and trapping performance. These results emphasize the importance of quantifying the effect of small-scale heterogeneity as they affect the large-scale behavior of the CO<span><math><mrow><msub><mrow></mrow><mrow><mn>2</mn></mrow></msub><mspace></mspace></mrow></math></span>plume.</div></div>","PeriodicalId":334,"journal":{"name":"International Journal of Greenhouse Gas Control","volume":"141 ","pages":"Article 104318"},"PeriodicalIF":4.6000,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"International Journal of Greenhouse Gas Control","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1750583625000167","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENERGY & FUELS","Score":null,"Total":0}
引用次数: 0
Abstract
Small-scale heterogeneities can significantly affect the fate of the plume and trapping during COmigration. We conducted geologic carbon storage field-scale simulations to investigate the impact of small-scale heterogeneities on plume dynamics and trapping performance. Small-scale heterogeneities have been shown to increase the amount of trapped COduring buoyancy-driven flow. The trapped saturation is validated by previous sandbox experimental work during buoyancy-driven flow in realistic heterogeneous domains and is implemented through the critical COsaturation parameter (i.e., the first non-zero value in the drainage COrelative permeability curve). Depending on the type and degree of heterogeneity, various critical COsaturation values are exhibited. Furthermore, we investigated the effect of small-scale heterogeneties when multiple capillary pressure models are employed. This study demonstrates that an increase in critical COsaturation reduces the COplume size and lateral extent, accompanying an increase in residual trapping and a decrease in solubility trapping. Finally, we show that independent of the capillary pressure model used, an increase in critical saturation leads to similar COplume dynamics distribution and trapping performance. These results emphasize the importance of quantifying the effect of small-scale heterogeneity as they affect the large-scale behavior of the COplume.
期刊介绍:
The International Journal of Greenhouse Gas Control is a peer reviewed journal focusing on scientific and engineering developments in greenhouse gas control through capture and storage at large stationary emitters in the power sector and in other major resource, manufacturing and production industries. The Journal covers all greenhouse gas emissions within the power and industrial sectors, and comprises both technical and non-technical related literature in one volume. Original research, review and comments papers are included.