Lithium-ion battery health estimate based on electrochemical impedance spectroscopy and CNN-BiLSTM-Attention

IF 2.6 4区 化学 Q3 CHEMISTRY, PHYSICAL Ionics Pub Date : 2024-12-13 DOI:10.1007/s11581-024-05982-8
Qingkai Xing, Xinwei Sun, Yaping Fu, Kai Wang
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Abstract

To ensure the safe operation and optimal performance of lithium battery systems, accurately determining the state of health (SOH) of the batteries is crucial. Research over the past few decades has shown that techniques based on electrochemical impedance spectroscopy (EIS) offer some advantages over traditional methods relying on voltage, current, and temperature. In this paper, we propose a novel approach for assessing the SOH of lithium-ion batteries using a CNN-BiLSTM-Attention model. By combining the effectiveness of bidirectional long short-term memory (BiLSTM) neural networks, known for their efficiency in long sequence prediction, with convolutional neural networks (CNN) capable of automatically extracting EIS features, we create a unique CNN-BiLSTM model. Additionally, an attention mechanism is incorporated to enhance the model’s accuracy and processing speed. This approach enables faster and more effective feature extraction while minimizing information loss from historical data. Experimental results demonstrate that the proposed model achieves higher estimation accuracy compared to other popular data-driven methods. When compared to the benchmark BiLSTM and CNN-BiLSTM models, the AC-BiLSTM model reduces the root mean squared error (RMSE) by 93.9% and 71.4%, respectively. These findings highlight the significant practical value of the proposed approach.

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基于电化学阻抗谱和cnn - bilstm的锂离子电池健康估计
为了确保锂电池系统的安全运行和最佳性能,准确确定电池的健康状态(SOH)至关重要。过去几十年的研究表明,与依赖电压、电流和温度的传统方法相比,基于电化学阻抗谱(EIS)的技术具有一些优势。在本文中,我们提出了一种使用CNN-BiLSTM-Attention模型来评估锂离子电池SOH的新方法。通过将双向长短期记忆(BiLSTM)神经网络(以其在长序列预测方面的效率而闻名)的有效性与能够自动提取EIS特征的卷积神经网络(CNN)相结合,我们创建了一个独特的CNN-BiLSTM模型。此外,还加入了注意机制,提高了模型的准确性和处理速度。这种方法可以更快、更有效地提取特征,同时最大限度地减少历史数据中的信息丢失。实验结果表明,与其他流行的数据驱动方法相比,该模型具有更高的估计精度。与基准BiLSTM和CNN-BiLSTM模型相比,AC-BiLSTM模型的均方根误差(RMSE)分别降低了93.9%和71.4%。这些发现突出了所提出的方法的重要实用价值。
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来源期刊
Ionics
Ionics 化学-电化学
CiteScore
5.30
自引率
7.10%
发文量
427
审稿时长
2.2 months
期刊介绍: Ionics is publishing original results in the fields of science and technology of ionic motion. This includes theoretical, experimental and practical work on electrolytes, electrode, ionic/electronic interfaces, ionic transport aspects of corrosion, galvanic cells, e.g. for thermodynamic and kinetic studies, batteries, fuel cells, sensors and electrochromics. Fast solid ionic conductors are presently providing new opportunities in view of several advantages, in addition to conventional liquid electrolytes.
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