Significantly energy-efficient ethanol sensor based on bougainvillea-like Au/ZnO hierarchical nanostructured materials

IF 2.3 4区 材料科学 Q2 MATERIALS SCIENCE, CERAMICS International Journal of Applied Ceramic Technology Pub Date : 2024-10-01 DOI:10.1111/ijac.14933
Ying Qi, Chengyou Liu, XiaoQi Yu, Zhaoxing Li, Hai Yu
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Abstract

The energy consumption of MOS (metal oxide semiconductor) sensors has always been a challenge in improving their performance. In this study, bougainvillea-like Au/ZnO nanostructures were successfully synthesized using the hydrothermal method and the sol fixation technique. The composition, crystallinity, crystal structure, and morphology of the materials were characterized using X-ray diffraction, energy-dispersive spectroscopy, and field emission scanning electron microscopy. The experimental results confirm the successful synthesis of a substantial quantity of bougainvillea-like Au/ZnO nanostructures through nanoparticle self-assembly. The sensitive performance of the bougainvillea-like Au/ZnO sensor was evaluated using a CGS-8 intelligent gas-sensitive analysis system. Results demonstrate that modification of ZnO with Au in a bougainvillea-like nanostructure significantly enhances sensitivity to ethanol vapor compared to those of unmodified material sensors. Specifically, the optimal work temperature was greatly reduced by 64%, whereas the sensitivity increased approximately 12 times and the response time decreased nearly 5 times. The significantly enhanced ethanol sensitivity can be attributed to the precious metal modification and unique three-dimensional morphology. It provides the necessary experimental exploration for reducing energy consumption and improving the performance of MOS gas sensors.

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基于九重葛状Au/ZnO层次化纳米结构材料的高效节能乙醇传感器
MOS(金属氧化物半导体)传感器的能耗问题一直是其性能提升的一大难题。本研究采用水热法和溶胶固定技术成功合成了九重葛状Au/ZnO纳米结构。利用x射线衍射、能量色散光谱和场发射扫描电镜对材料的组成、结晶度、晶体结构和形貌进行了表征。实验结果证实了通过纳米粒子自组装成功合成了大量的九重葛状Au/ZnO纳米结构。采用CGS-8智能气敏分析系统对九重梅类Au/ZnO传感器的灵敏性能进行了评价。结果表明,与未修饰的材料传感器相比,在九重葛状纳米结构中用Au修饰ZnO显著提高了对乙醇蒸汽的灵敏度。其中,最优工作温度降低了64%,灵敏度提高了约12倍,响应时间缩短了近5倍。乙醇敏感性的显著提高可归因于贵金属修饰和独特的三维形貌。为MOS气体传感器降低能耗和提高性能提供了必要的实验探索。
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来源期刊
International Journal of Applied Ceramic Technology
International Journal of Applied Ceramic Technology 工程技术-材料科学:硅酸盐
CiteScore
3.90
自引率
9.50%
发文量
280
审稿时长
4.5 months
期刊介绍: The International Journal of Applied Ceramic Technology publishes cutting edge applied research and development work focused on commercialization of engineered ceramics, products and processes. The publication also explores the barriers to commercialization, design and testing, environmental health issues, international standardization activities, databases, and cost models. Designed to get high quality information to end-users quickly, the peer process is led by an editorial board of experts from industry, government, and universities. Each issue focuses on a high-interest, high-impact topic plus includes a range of papers detailing applications of ceramics. Papers on all aspects of applied ceramics are welcome including those in the following areas: Nanotechnology applications; Ceramic Armor; Ceramic and Technology for Energy Applications (e.g., Fuel Cells, Batteries, Solar, Thermoelectric, and HT Superconductors); Ceramic Matrix Composites; Functional Materials; Thermal and Environmental Barrier Coatings; Bioceramic Applications; Green Manufacturing; Ceramic Processing; Glass Technology; Fiber optics; Ceramics in Environmental Applications; Ceramics in Electronic, Photonic and Magnetic Applications;
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