Lightweight spatial pyramid pooling convolutional neural network assisted hyperspectral imaging for Hangbaiju origin identification

IF 4.9 2区 化学 Q1 CHEMISTRY, ANALYTICAL Microchemical Journal Pub Date : 2025-01-01 Epub Date: 2024-12-01 DOI:10.1016/j.microc.2024.112352
Ming-Yue Dong , Wan-Jun Long , Hai-Long Wu , Tong Wang , Hai-Yan Fu , Kun Huang , Hang Ren , Ru-Qin Yu
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Abstract

Hangbaiju is a popular food supplement in the form of tea whose quality is influenced by the geographical origin. To control food quality, this work proposed a novel method, hyperspectral spatial pyramid pooling convolutional neural network (HSPPnet) assisted hyperspectral imaging (HSI), to identify the origin of Hangbaiju. HSPPnet utilizes both spatial and spectral information from hyperspectral images effectively and tolerates images of various sizes. This study initially evaluated the performance of four classical classification algorithms (k-NN, RF, XGBoost and PLS-DA) using hyperspectral average spectra, uncovering limitations in distinguishing samples with severe spectral overlap. Additionally, three representative deep learning models (VGG16, ResNet18, and DenseNet121) were used to analyze hyperspectral images compressed into three channels, resulting in overfitting due to the loss of detail information. Finally, HSPPnet and three improved deep learning models (VGG16-25, ResNet18-25, and DenseNet121-25) were used for Hangbaiju origin identification. HSPPnet achieved 100.0% accuracy for both the test set and prediction set, and three improved deep learning models also had been significantly improved. Through comparison, it was found that HSPPnet is an efficient and lightweight model, boasting the benefits of being faster, smaller, and more power-efficient. It was more suitable for deployment on HSI devices to realize large-scale inline detection. The interpretability of HSPPnet was studied to explore the pixel features of Hangbaiju hyperspectral images that were helpful for identification. Additionally, the proposed method exhibited excellent greenness and whiteness properties. The results showed that the proposed method was a non-destructive, efficient, and green method for Hangbaiju origin identification.

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轻量级空间金字塔池卷积神经网络辅助高光谱成像在杭白菊产地识别中的应用
杭白酒是一种受欢迎的以茶为形式的食品补充剂,其品质受地理产地的影响。为了控制食品质量,本文提出了一种新的方法——高光谱空间金字塔池卷积神经网络(HSPPnet)辅助高光谱成像(HSI)来鉴别杭白酒的产地。HSPPnet有效地利用了高光谱图像的空间和光谱信息,并能容忍各种尺寸的图像。本研究利用高光谱平均光谱初步评估了四种经典分类算法(k-NN、RF、XGBoost和PLS-DA)的性能,揭示了在区分严重光谱重叠样本方面的局限性。此外,使用三个具有代表性的深度学习模型(VGG16, ResNet18和DenseNet121)来分析压缩到三个通道的高光谱图像,由于细节信息的丢失而导致过拟合。最后,利用HSPPnet和3个改进的深度学习模型(VGG16-25、ResNet18-25和DenseNet121-25)对杭白酒进行产地识别。HSPPnet对测试集和预测集的准确率均达到100.0%,三个改进的深度学习模型也有显著提高。通过比较发现,HSPPnet是一种高效、轻量级的模型,具有更快、更小、更节能等优点。更适合部署在HSI器件上,实现大规模的内联检测。研究HSPPnet的可解释性,探索杭白居高光谱影像中有助于识别的像元特征。此外,该方法还具有良好的绿度和白度性能。结果表明,该方法是一种无损、高效、绿色的杭白酒产地鉴别方法。
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来源期刊
Microchemical Journal
Microchemical Journal 化学-分析化学
CiteScore
8.70
自引率
8.30%
发文量
1131
审稿时长
1.9 months
期刊介绍: The Microchemical Journal is a peer reviewed journal devoted to all aspects and phases of analytical chemistry and chemical analysis. The Microchemical Journal publishes articles which are at the forefront of modern analytical chemistry and cover innovations in the techniques to the finest possible limits. This includes fundamental aspects, instrumentation, new developments, innovative and novel methods and applications including environmental and clinical field. Traditional classical analytical methods such as spectrophotometry and titrimetry as well as established instrumentation methods such as flame and graphite furnace atomic absorption spectrometry, gas chromatography, and modified glassy or carbon electrode electrochemical methods will be considered, provided they show significant improvements and novelty compared to the established methods.
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