Analysis and Evaluation of Potential Adsorbent for CO2 Capture in a CI Engine Exhaust: An Experimental Study

IF 3 4区 环境科学与生态学 Q2 ENVIRONMENTAL SCIENCES Water, Air, & Soil Pollution Pub Date : 2025-02-05 DOI:10.1007/s11270-025-07780-y
Sushil Kumar Rathore, Maniarasu Ravi, Murugan Sivalingam
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Abstract

In this present study, initially, activated carbon is derived from eucalyptus wood utilizing a single-stage activation method. Then, the developed sample is characterized by different characterization and analytical techniques such as (i) proximate analysis, (ii) ultimate analysis, (iii) Brunauer–Emmett–Teller (BET) surface area analysis, (iv) Barrett-Joyner-Halenda (BJH) pore size analysis, (v) Scanning Electron Microscopy (SEM) surface morphology analysis, (vi) Fourier transform infrared spectroscopy (FTIR) surface chemistry analysis, and (vii) Thermogravimetric Analysis (TGA) thermal stability analysis to evaluate its surface features and ensure suitability as an adsorbent for carbon capture. After that, the characterized adsorbent is filled inside the capture unit and coupled to a test engine. This study uses a computerized diesel engine, and the test engine is operated by employing two distinct test fuels: (i) petro-diesel (D100) and (ii) 80% Jatropha methyl ester (JME) + 20% D100 (JME20). The adsorbent performance is examined in terms of CO2 adsorption, and the adsorbent sample’s adsorption parameter is discussed. The results obtained from experimental findings are compared with the adsorbent performance and fuels used in a test engine. The experimental test results showed that about 44% and 38% of CO2 emissions are captured for D100 and JME20 fuel operations, respectively.

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CI发动机废气中CO2捕集潜力吸附剂的分析与评价:实验研究
在本研究中,活性炭最初是利用单阶段活化法从桉树木材中提取的。然后,利用不同的表征和分析技术,如(i)近似分析,(ii)终极分析,(iii) brunauer - emmet - teller (BET)表面积分析,(iv) Barrett-Joyner-Halenda (BJH)孔径分析,(v)扫描电子显微镜(SEM)表面形貌分析,(vi)傅立叶变换红外光谱(FTIR)表面化学分析,热重分析(TGA)热稳定性分析,以评估其表面特征并确保其作为碳捕获吸附剂的适用性。之后,将所表征的吸附剂填充在捕获单元内并与测试发动机耦合。本研究使用计算机化柴油发动机,测试发动机使用两种不同的测试燃料:(i)石油柴油(D100)和(ii) 80%麻风树甲酯(JME) + 20% D100 (JME20)。从CO2吸附的角度考察了吸附剂的性能,并对吸附剂样品的吸附参数进行了讨论。并将实验结果与吸附剂性能及试验发动机上使用的燃料进行了比较。实验测试结果表明,D100和JME20燃料运行分别捕获了约44%和38%的CO2排放。图形抽象
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来源期刊
Water, Air, & Soil Pollution
Water, Air, & Soil Pollution 环境科学-环境科学
CiteScore
4.50
自引率
6.90%
发文量
448
审稿时长
2.6 months
期刊介绍: Water, Air, & Soil Pollution is an international, interdisciplinary journal on all aspects of pollution and solutions to pollution in the biosphere. This includes chemical, physical and biological processes affecting flora, fauna, water, air and soil in relation to environmental pollution. Because of its scope, the subject areas are diverse and include all aspects of pollution sources, transport, deposition, accumulation, acid precipitation, atmospheric pollution, metals, aquatic pollution including marine pollution and ground water, waste water, pesticides, soil pollution, sewage, sediment pollution, forestry pollution, effects of pollutants on humans, vegetation, fish, aquatic species, micro-organisms, and animals, environmental and molecular toxicology applied to pollution research, biosensors, global and climate change, ecological implications of pollution and pollution models. Water, Air, & Soil Pollution also publishes manuscripts on novel methods used in the study of environmental pollutants, environmental toxicology, environmental biology, novel environmental engineering related to pollution, biodiversity as influenced by pollution, novel environmental biotechnology as applied to pollution (e.g. bioremediation), environmental modelling and biorestoration of polluted environments. Articles should not be submitted that are of local interest only and do not advance international knowledge in environmental pollution and solutions to pollution. Articles that simply replicate known knowledge or techniques while researching a local pollution problem will normally be rejected without review. Submitted articles must have up-to-date references, employ the correct experimental replication and statistical analysis, where needed and contain a significant contribution to new knowledge. The publishing and editorial team sincerely appreciate your cooperation. Water, Air, & Soil Pollution publishes research papers; review articles; mini-reviews; and book reviews.
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