Shift of nanodroplet and nanocluster size distributions induced by dopant pick-up statistics.

IF 3.7 2区 化学 Q3 CHEMISTRY, PHYSICAL Journal of Chemical Physics Pub Date : 2025-02-07 DOI:10.1063/5.0252959
Marie Riddle, Angel I Pena Dominguez, Benjamin S Kamerin, Vitaly V Kresin
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Abstract

In pick-up experiments using nanodroplet and nanocluster beams, the size distribution of hosts carrying a specified number of dopants changes when the vapor density in the pick-up region is altered. This change, analyzed here, has quantitative consequences for the interpretation of data that are sensitive to host size, such as mass spectrometric, spectroscopic, and deflection measurements.

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掺杂量统计引起的纳米液滴和纳米团簇尺寸分布的变化。
在纳米液滴和纳米簇光束的吸积实验中,随着吸积区蒸汽密度的改变,携带一定数量掺杂剂的主体尺寸分布发生了变化。这里分析的这种变化对对宿主大小敏感的数据的解释有定量影响,例如质谱、光谱和偏转测量。
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来源期刊
Journal of Chemical Physics
Journal of Chemical Physics 物理-物理:原子、分子和化学物理
CiteScore
7.40
自引率
15.90%
发文量
1615
审稿时长
2 months
期刊介绍: The Journal of Chemical Physics publishes quantitative and rigorous science of long-lasting value in methods and applications of chemical physics. The Journal also publishes brief Communications of significant new findings, Perspectives on the latest advances in the field, and Special Topic issues. The Journal focuses on innovative research in experimental and theoretical areas of chemical physics, including spectroscopy, dynamics, kinetics, statistical mechanics, and quantum mechanics. In addition, topical areas such as polymers, soft matter, materials, surfaces/interfaces, and systems of biological relevance are of increasing importance. Topical coverage includes: Theoretical Methods and Algorithms Advanced Experimental Techniques Atoms, Molecules, and Clusters Liquids, Glasses, and Crystals Surfaces, Interfaces, and Materials Polymers and Soft Matter Biological Molecules and Networks.
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