Distribution and characteristics of Microplastics in leachate and underneath soil of two informal landfills

IF 7.1 2区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Waste management Pub Date : 2025-03-01 Epub Date: 2025-02-07 DOI:10.1016/j.wasman.2025.02.002
Jun Ma , Ming Ma , Jiangshan Li , Qirui Yang , Yong Wan , Kai Zhao , Yi Zhang , Lei Liu , Xunchang Fei
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Abstract

Microplastics (MPs), an emerging pollutant, have garnered global attention as significant environmental concerns. Landfills are the major sources of MPs. However, research on the distribution and characteristics of MPs in leachate and underneath soil of informal landfills remains limited. This study investigated the abundance, polymer type, size, and morphology of MPs in 6 leachate samples and 18 underneath soil samples at different depths from two informal landfills. The ranges of MPs abundance in leachate and underneath soil from landfills were 4,010–33,213 items/Land 592–870 to 47,819 items/kg, related to the landfilled waste composition. MPs size between 20 and 100 µm accounted for the highest proportion (70 %). The fragmentation coefficient α in the underneath soil was higher than that in the leachate, indicating smaller MPs were more likely to migrate into underneath soil after filtration. The fibrous MPs proportion was below 22 %, while the fragmented MPs was more than 78 %. Large fibrous MPs were detected in the underneath soil in landfill A. Polyethylene Terephthalate (PET), Polyurethane (PU) and Polystyrene (PS) were the predominant MPs polymers types in leachate and underneath soil. Polypropylene (PP) was primarily concentrated in the upper and middle underneath soil layers, and Polyurethane (PU) was predominantly in the middle and lower layers. Principal component analysis (PCA) results indicated that geographical factors significantly influenced the distribution and characteristics of MPs. This study revealed the distribution of MPs in leachate and underneath soil at different depths, providing a valuable reference for the risk assessment of MPs pollution.
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两个非正规填埋场渗滤液和土壤中微塑料的分布和特征
微塑料(MPs)作为一种新兴的污染物,已经引起了全球的关注。堆填区是MPs的主要来源。然而,对非正式填埋场渗滤液和地下土壤中MPs的分布和特征的研究仍然有限。本研究调查了两个非正式填埋场不同深度的6个渗滤液样品和18个地下土壤样品中MPs的丰度、聚合物类型、大小和形态。填埋场渗滤液和地下土壤中MPs丰度的变化范围为4010 ~ 33213个/kg,与填埋垃圾成分有关,592 ~ 870 ~ 47819个/kg。MPs尺寸在20 ~ 100µm之间的比例最高(70%)。土壤下部破碎系数α高于渗滤液,说明过滤后的MPs越小,越容易向土壤下部迁移。纤维状MPs的比例在22%以下,而碎片状MPs的比例在78%以上。垃圾填埋场地下土壤中检测到较大的纤维状MPs,其中,聚对苯二甲酸乙二醇酯(PET)、聚氨酯(PU)和聚苯乙烯(PS)是渗滤液和地下土壤中主要的MPs聚合物类型。聚丙烯(PP)主要集中在土层的上中层,聚氨酯(PU)主要集中在土层的中下层。主成分分析(PCA)结果表明,地理因素对MPs的分布和特征有显著影响。本研究揭示了不同深度下浸出液和土壤中MPs的分布情况,为MPs污染风险评价提供了有价值的参考。
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来源期刊
Waste management
Waste management 环境科学-工程:环境
CiteScore
15.60
自引率
6.20%
发文量
492
审稿时长
39 days
期刊介绍: Waste Management is devoted to the presentation and discussion of information on solid wastes,it covers the entire lifecycle of solid. wastes. Scope: Addresses solid wastes in both industrialized and economically developing countries Covers various types of solid wastes, including: Municipal (e.g., residential, institutional, commercial, light industrial) Agricultural Special (e.g., C and D, healthcare, household hazardous wastes, sewage sludge)
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