{"title":"Low-Contrast BIC Metasurfaces with Quality Factors Exceeding 100,000.","authors":"Keisuke Watanabe, Tadaaki Nagao, Masanobu Iwanaga","doi":"10.1021/acs.nanolett.4c05880","DOIUrl":null,"url":null,"abstract":"<p><p>Dielectric metasurfaces operating at quasi-bound states in the continuum (qBICs) can achieve exceptionally high radiative quality (<i>Q</i>) factors by introducing small asymmetries into their unit cells. However, fabrication imperfections often impose major limitations on the experimentally observed <i>Q</i> factors. In this study, we experimentally demonstrate BIC metasurfaces with a <i>Q</i> factor of 101,000 under normal excitation of light in the telecom wavelength range achieved by employing low-contrast silicon pairs. Our findings show that such free-space accessible ultrahigh-<i>Q</i> factors can be attained by leveraging both the high radiative <i>Q</i> factors of higher-order qBIC modes and reduced scattering losses in shallow-etched designs. Additionally, we demonstrate stable sub-picometer-level wavelength fluctuations in water, with a limit of detection of 10<sup>-5</sup> for environmental refractive index changes. The proposed approach can be extended to BIC metasurfaces with many other configurations and operating wavelengths for ultrahigh-<i>Q</i> applications in both fundamental physics and advanced devices.</p>","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":" ","pages":"2777-2784"},"PeriodicalIF":9.6000,"publicationDate":"2025-02-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano Letters","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acs.nanolett.4c05880","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2025/2/6 0:00:00","PubModel":"Epub","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Dielectric metasurfaces operating at quasi-bound states in the continuum (qBICs) can achieve exceptionally high radiative quality (Q) factors by introducing small asymmetries into their unit cells. However, fabrication imperfections often impose major limitations on the experimentally observed Q factors. In this study, we experimentally demonstrate BIC metasurfaces with a Q factor of 101,000 under normal excitation of light in the telecom wavelength range achieved by employing low-contrast silicon pairs. Our findings show that such free-space accessible ultrahigh-Q factors can be attained by leveraging both the high radiative Q factors of higher-order qBIC modes and reduced scattering losses in shallow-etched designs. Additionally, we demonstrate stable sub-picometer-level wavelength fluctuations in water, with a limit of detection of 10-5 for environmental refractive index changes. The proposed approach can be extended to BIC metasurfaces with many other configurations and operating wavelengths for ultrahigh-Q applications in both fundamental physics and advanced devices.
期刊介绍:
Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including:
- Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale
- Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies
- Modeling and simulation of synthetic, assembly, and interaction processes
- Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance
- Applications of nanoscale materials in living and environmental systems
Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.