Biodegradable air filter with electrospun composite nanofibers and cellulose fibers dual network: Enhanced electrostatic adsorption, humidity resistance, and extended service life

IF 11.3 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Journal of Hazardous Materials Pub Date : 2025-02-10 DOI:10.1016/j.jhazmat.2025.137557
Jingyi Nie, Binrong Sun, Tingting Jiao, Jianfei Liao, Meiyun Zhang, Ruiting Yang, Yueqing Li
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Abstract

Cellulose-based materials have great potential as degradable air filters. Regretfully, the application is limited by their low electrostatic adsorption and hydrophilicity. To meet with the challenge, we designed a composite air filter with dual network. Composite cellulose acetate nanofibers were electrospun on a cellulose-fibers paper substrate, and the resulted multi-scale spider-web-like structure showed high filtration efficiency as well as low resistance. Electrets (silicon nitride and tourmaline) were composited to enhance the electrostatic adsorption for PMs. Hydrophobic modification improved the ability to retain electrostatic charge, promoting the filtration under humid environment. The filtration efficiency for PM0.3 exceeded 99 %, while the pressure drop was only 45.7 Pa. The filtration performance could be maintained for over 12 hours under 90 % relative humidity, and the filter could be completely degraded in natural environment within 80 days.

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静电纺复合纳米纤维和纤维素纤维双重网络的可生物降解空气过滤器:增强静电吸附,抗湿性和延长使用寿命
纤维素基材料作为可降解空气过滤器具有很大的潜力。遗憾的是,其应用受到其低静电吸附和亲水性的限制。为了应对这一挑战,我们设计了一种双网复合空气过滤器。在纤维素-纤维纸基体上静电纺丝制备的复合醋酸纤维素纳米纤维具有高过滤效率和低过滤阻力的多尺度网状结构。利用氮化硅和电气石复合驻极体增强了pmms的静电吸附。疏水改性提高了静电电荷的保留能力,促进了潮湿环境下的过滤。对PM0.3的过滤效率超过99%,压降仅为45.7 Pa。在90%的相对湿度条件下,过滤性能可保持12小时以上,在自然环境下80天内可完全降解。
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产品信息
阿拉丁
N, N-dimethylacetamide
阿拉丁
Acetone
阿拉丁
Si3N4
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Tourmaline
阿拉丁
Methyltrimethoxysilane
来源期刊
Journal of Hazardous Materials
Journal of Hazardous Materials 工程技术-工程:环境
CiteScore
25.40
自引率
5.90%
发文量
3059
审稿时长
58 days
期刊介绍: The Journal of Hazardous Materials serves as a global platform for promoting cutting-edge research in the field of Environmental Science and Engineering. Our publication features a wide range of articles, including full-length research papers, review articles, and perspectives, with the aim of enhancing our understanding of the dangers and risks associated with various materials concerning public health and the environment. It is important to note that the term "environmental contaminants" refers specifically to substances that pose hazardous effects through contamination, while excluding those that do not have such impacts on the environment or human health. Moreover, we emphasize the distinction between wastes and hazardous materials in order to provide further clarity on the scope of the journal. We have a keen interest in exploring specific compounds and microbial agents that have adverse effects on the environment.
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