Plasmon Hot Carriers: Cognizing, Utilizing, and Regulating

IF 5.9 2区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY ChemSusChem Pub Date : 2025-02-09 DOI:10.1002/cssc.202402436
Wenkai Liang, Dong Li, Yawen Wang, Bo Zhao, Chang Liu, Yinghui Sun, Lin Jiang
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Abstract

The localized surface plasmon resonance (LSPR) effect can effectively utilize and transform solar energy, which is an ideal candidate to solve the energy crisis. In particular, plasmon hot carriers generated by LSPR effect are the focus of current research because their energy characteristics are higher than the Fermi level, which can easily promote the chemical reaction on the catalysts and improve the photoelectric performance of the optoelectronic devices. In this review, the generation of hot carriers and their decay pathways under different nano-structured models are discussed, and their unique significance is highlighted. Meanwhile, recent research advances in cognizing the plasmon hot carriers, the role of hot carriers in various applications, and the regulating mechanism of hot carriers in the nanostructure are discussed in depth. In addition, the limitations and challenges of the current research on plasmon hot carriers are presented, and prospects for the future are proposed.

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等离子体热载流子:认识、利用与调控。
局域表面等离子体共振(LSPR)效应可以有效地利用和转化太阳能,是解决能源危机的理想选择。特别是由LSPR效应产生的等离子体热载子,由于其能量特性高于费米能级,容易促进催化剂上的化学反应,提高光电器件的光电性能,成为当前研究的热点。本文综述了热载流子的产生及其在不同纳米结构模型下的衰变途径,并强调了其独特的意义。同时,对等离子体热载流子的认识、热载流子在各种应用中的作用以及热载流子在纳米结构中的调控机制等方面的最新研究进展进行了深入讨论。此外,还指出了等离子体热载流子研究的局限性和面临的挑战,并对未来的研究进行了展望。
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来源期刊
ChemSusChem
ChemSusChem 化学-化学综合
CiteScore
15.80
自引率
4.80%
发文量
555
审稿时长
1.8 months
期刊介绍: ChemSusChem Impact Factor (2016): 7.226 Scope: Interdisciplinary journal Focuses on research at the interface of chemistry and sustainability Features the best research on sustainability and energy Areas Covered: Chemistry Materials Science Chemical Engineering Biotechnology
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