Nonreciprocal Metasurfaces with Epsilon-Near-Zero Materials

IF 9.6 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Nano Letters Pub Date : 2025-02-12 DOI:10.1021/acs.nanolett.4c06188
Albert Mathew, Rebecca Aschwanden, Aditya Tripathi, Piyush Jangid, Basudeb Sain, Thomas Zentgraf, Sergey Kruk
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Abstract

Nonreciprocal optics enables the asymmetric transmission of light when its sources and detectors are exchanged. A canonical example─optical isolator─enables light propagation in only one direction, similar to how electrical diodes enable unidirectional flow of electric current. Nonreciprocal optics today, unlike nonreciprocal electronics, remains bulky. Recently, nonlinear metasurfaces opened a pathway to strong optical nonreciprocity on the nanoscale. However, demonstrations to date were based on optically slow nonlinearities involving thermal effects or phase transition materials. In this work, we demonstrate a nonreciprocal metasurface with an ultrafast optical response based on indium tin oxide in its epsilon-near-zero regime. It operates in the spectral range of 1200–1300 nm with incident power densities of 40–70 GW/cm2. Furthermore, the nonreciprocity of the metasurface extends to both amplitude and phase of the forward/backward transmission, opening a pathway to nonreciprocal wavefront control at the nanoscale.

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当光源和探测器交换时,非互易光学可实现光的非对称传输。一个典型的例子--光隔离器--只允许光在一个方向上传播,类似于二极管允许电流单向流动。如今的非互易光学与非互易电子学不同,仍然十分笨重。最近,非线性元表面开辟了在纳米尺度上实现强光学非互易性的途径。然而,迄今为止的演示都是基于涉及热效应或相变材料的光学慢非线性。在这项研究中,我们展示了一种具有超快光学响应的非互易元表面,它基于ε-近零状态下的氧化铟锡。它的工作光谱范围为 1200-1300 nm,入射功率密度为 40-70 GW/cm2。此外,元表面的非互易性还扩展到了前向/后向传输的振幅和相位,为纳米级非互易波前控制开辟了道路。
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来源期刊
Nano Letters
Nano Letters 工程技术-材料科学:综合
CiteScore
16.80
自引率
2.80%
发文量
1182
审稿时长
1.4 months
期刊介绍: Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including: - Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale - Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies - Modeling and simulation of synthetic, assembly, and interaction processes - Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance - Applications of nanoscale materials in living and environmental systems Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.
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