Formation and Evolution of Complex Pore-Fracture Systems in Shale Gas Reservoirs: Insights into Controlling Mechanisms

IF 5.3 3区 工程技术 Q2 ENERGY & FUELS Energy & Fuels Pub Date : 2025-02-05 DOI:10.1021/acs.energyfuels.4c05306
Haodong Hou, Wei Yang*, Rui Yang*, Zhenxue Jiang, Ke Miao, Weihao Sun and Yating Xiao, 
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Abstract

Lacustrine fine-grained sedimentary rocks exhibit various lithofacies types and strong multiscale heterogeneity, encouraging us to investigate multistage characteristics of the panoramic pore-microfracture evolution process and potential triggering mechanisms of continental shale reservoirs. We present new results here from organic geochemistry analysis, X-ray diffraction, total organic carbon (TOC) analysis, the R0 test, rock pyrolysis analysis, field emission scanning electron microscopy, low-pressure CO2 and N2 adsorption, high-pressure mercury injection (MIP), nuclear magnetic resonance (NMR), and spontaneous imbibition tests. First, we conducted thermal simulation experiments using low-mature shale samples with an R0 value of 0.67%, aiming to innovatively unravel the entire dynamic evolution process of the micropore-fracture system in continental shales. Multitemperature thermal simulation investigations on naturally low-mature shale samples show that (1) the extensively developed interparticle pores and microfractures are conducive to the formation of complex and heterogeneous pore-fracture network systems. (2) The multistage evolution process of the pore-fracture system in continental shale reservoirs is triggered by differential hydrocarbon generation potential of maceral components, clay mineral transformation, and catalysis processes. (3) Four stages of the pore-fracture system evolution of the shale reservoir were identified, respectively occurring in R0 ≤ 0.9, 0.9% < R0 ≤ 1.6, 1.6% < R0 ≤ 3.0%, and R0 > 3.0%. This study laid a foundation for future research into differential diagenetic and reservoir-forming mechanisms of continental shale reservoirs, offering new insights into accurate prediction and comprehensive evaluation of the lacustrine shale gas “sweet spot”.

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页岩气储层复杂孔隙-裂缝系统的形成与演化:控制机制
湖相细粒沉积岩具有丰富的岩相类型和较强的多尺度非均质性,为研究陆相页岩储集层全景孔隙-微裂缝演化过程的多阶段特征和潜在的触发机制提供了理论依据。本文介绍了有机地球化学分析、x射线衍射、总有机碳(TOC)分析、R0测试、岩石热解分析、场发射扫描电镜、低压CO2和N2吸附、高压压汞(MIP)、核磁共振(NMR)和自发渗吸试验的新结果。首先,采用R0值为0.67%的低成熟页岩样品进行热模拟实验,创新性地揭示了陆相页岩微孔-裂缝系统的整个动态演化过程。对天然低成熟页岩样品的多温热模拟研究表明:(1)广泛发育的粒间孔隙和微裂缝有利于形成复杂非均质孔缝网络系统。(2)陆相页岩储层孔隙-裂缝系统的多阶段演化过程是由显微组分的差异生烃潜力、粘土矿物转化和催化作用等共同引发的。(3)识别出页岩储层孔隙-裂缝系统演化的4个阶段,分别发生在R0≤0.9、0.9% <;R0≤1.6,1.6% <;R0≤3.0%,R0 >;3.0%。该研究为进一步开展陆相页岩储层差异成岩成藏机制研究奠定了基础,为湖相页岩气“甜点”的准确预测和综合评价提供了新思路。
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来源期刊
Energy & Fuels
Energy & Fuels 工程技术-工程:化工
CiteScore
9.20
自引率
13.20%
发文量
1101
审稿时长
2.1 months
期刊介绍: Energy & Fuels publishes reports of research in the technical area defined by the intersection of the disciplines of chemistry and chemical engineering and the application domain of non-nuclear energy and fuels. This includes research directed at the formation of, exploration for, and production of fossil fuels and biomass; the properties and structure or molecular composition of both raw fuels and refined products; the chemistry involved in the processing and utilization of fuels; fuel cells and their applications; and the analytical and instrumental techniques used in investigations of the foregoing areas.
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