All chemically fabricated Co-Pt nanoparticle spin thermoelectric generator on plastic sheet

Yuichiro Kurokawa , Keisuke Yamada , Kenji Tanabe , Hideki Matsui , Hiromi Yuasa
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Abstract

The anomalous Nernst effect (ANE) is a heat-charge conversion phenomenon based on magnetic metals that has been extensively studied for use in thermoelectric power generators and heat flow sensors. Thermoelectric power-generation devices require flexibility to accommodate a wide range of applications. In this study, we fabricated a thermoelectric power generator using Co-Pt nanoparticles (NPs) on plastic sheets via a chemical process. The ANE voltage in the Co-Pt NP-assembled film could be successfully observed. Additionally, the thermal conductivity of the NP-assembled film was lower than that of the thin film, owing to the large number of grain boundaries and voids that can scatter phonons. This is important for practical applications because the thermoelectric figure of merit is inversely proportional to thermal conductivity. These results indicate that Co-Pt NP-assembled films are promising materials because they suggest that a thermoelectric generator based on ANE can be fabricated using simple chemical processes that are advantageous for commercial use.
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全化学制造的钴铂纳米粒子自旋热电发电机在塑料片
反常能效应(ANE)是一种基于磁性金属的热荷转换现象,已被广泛研究用于热电发电机和热流传感器。热电发电设备需要灵活性,以适应广泛的应用。在这项研究中,我们利用Co-Pt纳米颗粒(NPs)在塑料片上通过化学工艺制造了热电发电机。可以成功地观察到Co-Pt np组装膜中的ANE电压。此外,由于大量的晶界和可以散射声子的空隙,np组装膜的导热系数比薄膜低。这对实际应用很重要,因为热电性能与导热系数成反比。这些结果表明,Co-Pt np组装薄膜是很有前途的材料,因为它们表明,基于ANE的热电发电机可以使用简单的化学工艺制造,有利于商业用途。
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