Flame-Free Candles Are Not Pollution-Free: Scented Wax Melts as a Significant Source of Atmospheric Nanoparticles.

Abstract

Scented wax melts are being popularized as a safer, nontoxic alternative to traditional candles and incense for indoor aromatherapy. We performed field measurements in a residential test house to investigate atmospheric nanoparticle formation from scented wax melt use. We employed a high-resolution particle size magnifier-scanning mobility particle sizer (PSMPS) and a proton transfer reaction time-of-flight mass spectrometer (PTR-TOF-MS) for real-time monitoring of indoor atmospheric nanoparticle size distributions and terpene mixing ratios, respectively. Our findings reveal that terpenes released from scented wax melts react with indoor atmospheric ozone (O₃) to initiate new particle formation (NPF) events, resulting in significant indoor atmospheric nanoparticle concentrations (>10⁶ cm^-3) comparable to those emitted by combustion-based scented candles, gas stoves, diesel engines, and natural gas engines. We show that scented wax melt-initiated NPF events can result in significant respiratory exposures, with nanoparticle respiratory tract deposited dose rates similar to those determined for combustion-based sources. Our results challenge the perception of scented wax melts as a safer alternative to combustion-based aromatherapy, highlighting the need for further research on the toxicological properties of the newly formed nanoparticles to better understand their environmental health implications.