Soil heavy metals assessment of the Zhoukou riparian zone base of Shaying river basin, China: spatial distribution, source analysis and ecological risk.

IF 3.8 3区 环境科学与生态学 Q3 ENGINEERING, ENVIRONMENTAL Environmental Geochemistry and Health Pub Date : 2025-02-17 DOI:10.1007/s10653-025-02391-2
Yimei Ying, Meng Shang, Xu Wang, Xinrui Cui, Ruijie Huang, Zhixin Song, Yunjiao Han
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Abstract

The riparian zone serves as an ecological transition area between aquatic and terrestrial environments. Understanding the spatial distribution and origins of heavy metals within this zone is crucial for studying riverine ecosystems. In this research, we assessed the occurrence forms and spatial patterns of heavy metals in the riparian zone of the Shaying River Basin in Zhoukou City. Environmental risks were preliminarily evaluated using indices such as Igeo, RI, and PLI, and the sources of heavy metals were identified through PMF. The results revealed that the overall ecological risk associated with eight analyzed heavy metals (Cd, Co, Cr, Cu, Mn, Ni, Pb, Zn) in this region was low. However, Cd is marked enriched and represents a significant factor contributing to the potential ecological risk within the riparian zone of the basin. The high bioavailability of Cd and Mn in the soils of nine more contaminated sites showed moderate to very high ecological risk. The PMF model identified four pollution primary sources in this region: agricultural and industrial activities (29.4%), upstream water pollution (21.1%), natural sources (26.5%), and transport-related source (23.1%). These findings establish a scientific foundation for the conservation and management of the ecological environment in the riparian zone of the Shaying River Basin in Zhoukou City. Additionally, they will serve as a reference for future research on soil heavy metal migration and sources within the Huaihe River Basin, China.

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沙营河流域周口河岸带基地土壤重金属评价:空间分布、来源分析与生态风险
河岸带是水生环境和陆生环境之间的生态过渡区。了解该区域重金属的空间分布和来源对研究河流生态系统至关重要。本文对周口市沙营河流域河岸带重金属赋存形态及空间格局进行了评价。利用Igeo、RI、PLI等指标对环境风险进行初步评价,并通过PMF对重金属来源进行识别。结果表明,8种重金属(Cd、Co、Cr、Cu、Mn、Ni、Pb、Zn)对该区的总体生态风险较低。然而,Cd明显富集,是造成流域河岸带潜在生态风险的重要因素。另外9个污染点土壤Cd和Mn的生物有效性较高,显示出中度至极高的生态风险。PMF模型确定了该地区的4个主要污染源:农业和工业活动(29.4%)、上游水污染(21.1%)、自然污染源(26.5%)和运输相关污染源(23.1%)。研究结果为周口市沙营河流域河岸带生态环境的保护与管理提供了科学依据。为今后淮河流域土壤重金属迁移及来源研究提供参考。
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来源期刊
Environmental Geochemistry and Health
Environmental Geochemistry and Health 环境科学-工程:环境
CiteScore
8.00
自引率
4.80%
发文量
279
审稿时长
4.2 months
期刊介绍: Environmental Geochemistry and Health publishes original research papers and review papers across the broad field of environmental geochemistry. Environmental geochemistry and health establishes and explains links between the natural or disturbed chemical composition of the earth’s surface and the health of plants, animals and people. Beneficial elements regulate or promote enzymatic and hormonal activity whereas other elements may be toxic. Bedrock geochemistry controls the composition of soil and hence that of water and vegetation. Environmental issues, such as pollution, arising from the extraction and use of mineral resources, are discussed. The effects of contaminants introduced into the earth’s geochemical systems are examined. Geochemical surveys of soil, water and plants show how major and trace elements are distributed geographically. Associated epidemiological studies reveal the possibility of causal links between the natural or disturbed geochemical environment and disease. Experimental research illuminates the nature or consequences of natural or disturbed geochemical processes. The journal particularly welcomes novel research linking environmental geochemistry and health issues on such topics as: heavy metals (including mercury), persistent organic pollutants (POPs), and mixed chemicals emitted through human activities, such as uncontrolled recycling of electronic-waste; waste recycling; surface-atmospheric interaction processes (natural and anthropogenic emissions, vertical transport, deposition, and physical-chemical interaction) of gases and aerosols; phytoremediation/restoration of contaminated sites; food contamination and safety; environmental effects of medicines; effects and toxicity of mixed pollutants; speciation of heavy metals/metalloids; effects of mining; disturbed geochemistry from human behavior, natural or man-made hazards; particle and nanoparticle toxicology; risk and the vulnerability of populations, etc.
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