Origin of Water and Hydrochemical Components of Lakes: Example From the Mu Us Desert, Northwest China

IF 5 1区 地球科学 Q2 ENVIRONMENTAL SCIENCES Water Resources Research Pub Date : 2025-02-19 DOI:10.1029/2024wr038856
Fengxia Liu, Guangcai Wang, Fu Liao, Zheming Shi, Charles Cravotta, Pengpeng Zhou, Xiangyang Liang
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Abstract

Desert lakes are sparsely distributed in arid/semi-arid regions of the world and are crucial to desert hydro-ecosystem. However, the sources of water and dissolved components in desert lakes, especially the inputs from anthropogenic activities, remain to be fully understood. This study used water stable isotopes, self-organizing maps, and principal component analysis to explore the origins of lake water in the Mu Us desert, northwest China, where intensive coal mining activities exist. Results show that all desert lakes were distinguished into two types: (a) Type A, dominated by Ca-HCO3 type with a relatively low TDS (192–405 mg/L) and the highest concentration of NO3 (1.14–5.94 mg/L); (b) Type B, characterized by Na-HCO3 type with a highest content of SO42– and TDS up to 159 and 1,207 mg/L, respectively. The water stable isotopic compositions in lake water of Type B are depleted compared to those of the lake water of Type A. A combined analysis of hydrochemistry of lake water, groundwater, and mine water suggest that the desert lakes have different sources: lake water of Type A originated from Quaternary groundwater discharge, while lake water of Type B was derived from the treated mine drainage (TMD) which led to higher TDS and SO42–. The hydrochemistry of Type A lakes was influenced by agricultural activities (fertilizer use and livestock manure), whereas the hydrochemistry in Type B lakes were mainly controlled by the infiltrated TMD nearby. This hydrochemical characterization approach may be helpful to understand the hydrology of desert lakes elsewhere.
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湖泊水的成因及水化学成分——以中国西北毛乌素沙漠为例
沙漠湖泊在世界干旱/半干旱地区分布稀少,对沙漠水文生态系统至关重要。但是,沙漠湖泊的水和溶解成分的来源,特别是人类活动的投入,仍有待充分了解。本研究利用水稳定同位素、自组织图和主成分分析等方法,探讨了中国西北毛乌素沙漠湖泊水的来源。结果表明:(a) a型以Ca-HCO3型为主,TDS较低(192 ~ 405 mg/L), NO3−浓度最高(1.14 ~ 5.94 mg/L);(b) b型,为Na-HCO3型,SO42 -和TDS含量最高,分别为159和1207 mg/L。B型湖泊的水稳定同位素组成比A型湖泊的水稳定同位素组成低。结合湖泊、地下水和矿山水的水化学分析表明,A型湖泊的水来源于第四纪地下水排放,而B型湖泊的水来源于处理过的矿山水(TMD),导致其TDS和SO42 -含量较高。A类湖泊的水化学主要受农业活动(肥料使用和畜禽粪便)的影响,而B类湖泊的水化学主要受附近渗透的TMD控制。这种水化学表征方法可能有助于了解其他地方沙漠湖泊的水文。
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来源期刊
Water Resources Research
Water Resources Research 环境科学-湖沼学
CiteScore
8.80
自引率
13.00%
发文量
599
审稿时长
3.5 months
期刊介绍: Water Resources Research (WRR) is an interdisciplinary journal that focuses on hydrology and water resources. It publishes original research in the natural and social sciences of water. It emphasizes the role of water in the Earth system, including physical, chemical, biological, and ecological processes in water resources research and management, including social, policy, and public health implications. It encompasses observational, experimental, theoretical, analytical, numerical, and data-driven approaches that advance the science of water and its management. Submissions are evaluated for their novelty, accuracy, significance, and broader implications of the findings.
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