Comprehensive performance investigation of the novel mixed flow field for proton exchange membrane fuel cells: Three-dimensional multiphase simulation of a full-scale cell

IF 3.8 3区 工程技术 Q3 ENERGY & FUELS Chemical Engineering and Processing - Process Intensification Pub Date : 2025-02-17 DOI:10.1016/j.cep.2025.110234
Fan Fan , Meng Gu , Yangyang Chen , Dongjian Zhang , Haoyan Fang , Baofeng Hu , Yong Zhang , Qingshan Liu
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Abstract

This study addresses the challenges associated with proton exchange membrane fuel cells, specifically focusing on the bipolar plates which often suffer from weak mass transfer capabilities, significant pressure losses, and uneven internal liquid distribution. Initially, the research explores the advantages and disadvantages inherent in single-channel serpentine flow fields and interdigitated flow fields. By integrating these two configurations, a novel mixed flow field (MFF) is developed to enhance the output performance of fuel cells while maintaining consistent water distribution within the porous electrodes. Subsequently, an experimental test platform for a single cell is established. It is observed that the experimental results are slightly lower than the simulations, particularly in the ohmic voltage loss region. Further investigation is conducted into the impact of inlet/outlet arrangements of the MFF on the comprehensive characteristics of the cell, and the third arrangement method demonstrates optimal uniformity in membrane water content distribution. Finally, the study examines the macroscopic performance characteristics and spatial distribution of various physical quantities of the MFF under different operating conditions, such as cathode inlet humidity and operating voltage. The findings indicate that the MFF exhibits optimal comprehensive output performance at an inlet humidity of 60 % and an operating voltage of 0 .5V.

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本研究探讨了质子交换膜燃料电池所面临的挑战,特别是双极板通常存在传质能力弱、压力损失大和内部液体分布不均匀等问题。研究首先探讨了单通道蛇形流场和交错流场固有的优缺点。通过整合这两种配置,开发出一种新型混合流场 (MFF),以提高燃料电池的输出性能,同时保持多孔电极内水分布的一致性。随后,建立了单个电池的实验测试平台。据观察,实验结果略低于模拟结果,尤其是在欧姆电压损失区域。研究还进一步探究了 MFF 的入口/出口布置对电池综合特性的影响,第三种布置方法展示了膜含水量分布的最佳均匀性。最后,研究考察了 MFF 在阴极入口湿度和工作电压等不同工作条件下的宏观性能特征和各种物理量的空间分布。研究结果表明,在入口湿度为 60%、工作电压为 0.5V 的条件下,MFF 的综合输出性能最佳。
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来源期刊
CiteScore
7.80
自引率
9.30%
发文量
408
审稿时长
49 days
期刊介绍: Chemical Engineering and Processing: Process Intensification is intended for practicing researchers in industry and academia, working in the field of Process Engineering and related to the subject of Process Intensification.Articles published in the Journal demonstrate how novel discoveries, developments and theories in the field of Process Engineering and in particular Process Intensification may be used for analysis and design of innovative equipment and processing methods with substantially improved sustainability, efficiency and environmental performance.
期刊最新文献
Intensification and enhancement of phenolic compounds extraction using cooperative formulation Editorial Board Enhanced chloroquine adsorption using cobalt-modified mesoporous silicas for water treatment Comprehensive performance investigation of the novel mixed flow field for proton exchange membrane fuel cells: Three-dimensional multiphase simulation of a full-scale cell Development of 3D-printed electrodes using polyacrylonitrile/ graphene composites for application in polysulfide bromide flow battery
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