Performance evaluation of organometal halide MASnI3 and inorganic BaZrS3 hybrids in perovskites solar cells: Theoretical approach

Hybrid Advances Pub Date : 2025-02-17 DOI:10.1016/j.hybadv.2025.100408

Syed M. Hasnain , Abid Iqbal , Irfan Qasim , Kamran Irshad , M. Amin Mir , Muhammad Imran Malik , L. Syam Sundar

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Abstract

Perovskite solar cells have made substantial progress in efficiency and technology for the future photovoltaic systems. Study investigates effect of absorber layer composition on effectiveness power conversion efficiency of solar cell configured with ITO/ZnO/MASnI₃/CuSCN/Au and ITO/ZnO/BaZrS₃/CuSCN/Au material. Using SCAPS-1D simulation tool, the optimized structural layer thicknesses, maximize device efficiency was analyzed. The MASnI₃-based perovskite solar cells consistently outperformed their BaZrS₃ counterparts, with optimized thicknesses of 0.03 μm for the ZnO layer and 0.8 μm for the MASnI₃ absorber layer, yielding a PCE of 20.17 %, an open-circuit voltage (V_oc) of 0.8378 V, a short-circuit current density (J_sc) of 34.18 mA/cm² and a fill factor (FF) of 70.45 %. Conversely, the BaZrS₃-based cells, with optimal thicknesses of 0.04 μm for the ZnO layer and 0.50 μm for the BaZrS₃ absorber layer, achieved a PCE of 8.28 %, a V_oc of 1.3758 V, a J_sc of 13.92 mA/cm², and an FF of 43.24 %.

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Hybrid Advances

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