Anomalous temperature dependence of spin-orbit coupling in Al2O3/SrTiO3and Al2O3/KTaO3heterostructures.

IF 2.6 4区 物理与天体物理 Q3 PHYSICS, CONDENSED MATTER Journal of Physics: Condensed Matter Pub Date : 2025-03-03 DOI:10.1088/1361-648X/adb924
Z Qin, D B Zhou, X R Ma, T Lin, K H Gao
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Abstract

Perovskite oxide-based heterostructures exhibit a range of exotic physical properties such as two-dimensional superconductivity, interface magnetism, tunable Kondo effect, and tunable spin-orbit coupling. Here, the magnetotransport properties of Al2O3/SrTiO3and Al2O3/KTaO3heterostructures are studied. Both Kondo effect and spin-orbit coupling-induced weak antilocalization (WAL) effect are observed at low temperatures. By analyzing the WAL curves, the spin relaxation time is extracted. Surprisingly, the extracted spin relaxation time unexpectedly decreases on increasing temperature in all samples. This indicates that the strength of the spin-orbit coupling is progressively enhanced on increasing temperature, conflicting with theoretical prediction. This anomalous temperature dependence is explained by the interplay between the Kondo effect and the D'yakonov-Perel spin relaxation mechanism.

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Al2O3/SrTiO3和Al2O3/KTaO3异质结构中自旋轨道耦合的反常温度依赖性
基于钙钛矿氧化物的异质结构表现出一系列奇异的物理性质,如二维超导性、界面磁性、可调谐近藤效应和可调谐自旋轨道耦合。本文研究了Al2O3/SrTiO3和Al2O3/KTaO3异质结构的磁输运特性。在低温下观察到近藤效应和自旋轨道耦合引起的弱反局域化效应。通过分析WAL曲线,提取了自旋弛豫时间。令人惊讶的是,在所有样品中,提取的自旋弛豫时间出乎意料地随温度的升高而降低。这表明自旋轨道耦合的强度随着温度的升高而逐渐增强,这与理论预测相矛盾。这种反常的温度依赖性可以用近藤效应和D'yakonov-Perel自旋弛豫机制之间的相互作用来解释。
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来源期刊
Journal of Physics: Condensed Matter
Journal of Physics: Condensed Matter 物理-物理:凝聚态物理
CiteScore
5.30
自引率
7.40%
发文量
1288
审稿时长
2.1 months
期刊介绍: Journal of Physics: Condensed Matter covers the whole of condensed matter physics including soft condensed matter and nanostructures. Papers may report experimental, theoretical and simulation studies. Note that papers must contain fundamental condensed matter science: papers reporting methods of materials preparation or properties of materials without novel condensed matter content will not be accepted.
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