All-in-One PANI@PDA/PVDF Smart Textiles for Multifunctional Biomonitoring

IF 4.7 3区 材料科学 Q1 ENGINEERING, ELECTRICAL & ELECTRONIC ACS Applied Electronic Materials Pub Date : 2025-02-16 DOI:10.1021/acsaelm.4c02132
Haozhen Li, Shangling Yang, Guangzhong Xie* and Yuanjie Su*, 
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Abstract

Smart textiles play a vital role in physiological monitoring, mobile healthcare, and human–machine interface. Multifunctionality remarkably benefits the miniaturization and integration of wearable electronics. Here, we developed a PANI@PDA/PVDF composite textile (PCT)-based multifunctional sensor by combining electrospinning with in situ polymerization. This prepared multifunctional sensor features a wide pressure detection range (0–70 kPa), high sensitivity (10.1 [kPa]−1), fast response rate, and excellent stability, which is capable of discerning subtle pulse, respiratory patterns, and limb movement. Furthermore, the PDA anchoring-enabled π–π conjugation effect promises good ammonia sensing performance with a sensitivity of 1.76% ppm–1 and a response of 320.5% at 200 ppm of NH3, demonstrating great potential in distinguishing the biomarker for kidney disease prognosis. This work unravels the possibility for constructing multifunctional biomonitoring devices for multimodal physiological diagnosis.

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多功能生物监测用全合一PANI@PDA/PVDF智能纺织品
智能纺织品在生理监测、移动医疗和人机界面方面发挥着至关重要的作用。多功能性显著地有利于可穿戴电子产品的小型化和集成化。本文采用静电纺丝和原位聚合相结合的方法,研制了一种基于PANI@PDA/PVDF复合纺织品(PCT)的多功能传感器。该多功能传感器具有压力检测范围宽(0-70 kPa)、灵敏度高(10.1 [kPa]−1)、响应速度快、稳定性好等特点,能够识别细微的脉搏、呼吸模式和肢体运动。此外,PDA锚定激活的π -π偶联效应保证了良好的氨传感性能,灵敏度为1.76% ppm - 1,在200ppm NH3下的响应率为320.5%,在区分肾脏疾病预后的生物标志物方面具有很大的潜力。这项工作揭示了构建多功能生物监测设备用于多模式生理诊断的可能性。
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来源期刊
CiteScore
7.20
自引率
4.30%
发文量
567
期刊介绍: ACS Applied Electronic Materials is an interdisciplinary journal publishing original research covering all aspects of electronic materials. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials science, engineering, optics, physics, and chemistry into important applications of electronic materials. Sample research topics that span the journal's scope are inorganic, organic, ionic and polymeric materials with properties that include conducting, semiconducting, superconducting, insulating, dielectric, magnetic, optoelectronic, piezoelectric, ferroelectric and thermoelectric. Indexed/​Abstracted: Web of Science SCIE Scopus CAS INSPEC Portico
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