Kirigami-Inspired Light-Responsive Conical Spiral Actuators with Large Contraction Ratio Using Liquid Crystal Elastomer Fiber

Abstract

Liquid crystal elastomers (LCEs) are among the key smart materials driving soft robotics and LCE fibers have garnered significant attention for their rapid response characteristics. A convenient and fast method for programming orientations of liquid crystal molecules is a focal issue in LCE applications. Inspired by the Kirigami technique, here, we propose a novel method for fabricating LCE fibers based on customizable cutting paths and secondary photo-cross-linking. While most existing LCE actuators exhibit contraction ratios of around 30 to 40%, our conical spiral actuator, fabricated from LCE-carbon nanotube (CNT) fiber using the proposed method, demonstrates a significantly higher contraction ratio, reaching up to 80%. The contraction ratio can be controlled by adjusting the cutting path parameters and we elucidate the mechanism linking liquid crystal orientation to the distribution of contraction ratio. Additionally, the conical spiral deformation of the actuator can be manipulated with light radiation, enabling versatile functionalities such as catching, twisting, and gripping. We hope that the novel LCE fiber fabrication method presented provides new insights for programming and preparing LCE fibers, offering a valuable reference for the application of smart soft materials.