Femtosecond laser induced periodic subwavelength nanohole arrays structure on As2Se3 glass surface

IF 5.6 2区材料科学 Q1 MATERIALS SCIENCE, CERAMICS Ceramics International Pub Date : 2025-03-01 DOI:10.1016/j.ceramint.2024.12.302

Zhanzhu Li , Shiyong Shangguan , Wei Shi , Wenke Wang , Dongfeng Qi , Feifei Chen , Hongyu Zheng

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Abstract

The phenomenon of laser-induced periodic surface structures (LIPSS) evolution on As₂Se₃ was investigated through femtosecond laser irradiation. In this experiment, the periodic surface structure (LIPSS) is manipulated by controlling the number of pulses, ultimately achieving precise fabrication of nanopore arrays. The numerical simulation of the time-domain finite-difference technique was used to reveal the mechanism of evolution. We found that the initial formation of low-spatial frequency LIPSS (LSFL) gratings would change the distribution of the electric field and play a crucial role in the generation of subsequent nanohole arrays. One-to five-row nanohole array was prepared on the As₂Se₃ surface by varying the scanning speed of femtosecond laser direct writing. We have shown that the nanoholes' overall and individual morphology trends confirm the significance of the initial gratings on the subsequent structure. Finally, the large-area nanohole array prepared on the As₂Se₃ surface shows an excellent application in the structural color.

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飞秒激光诱导As2Se3玻璃表面的周期性亚波长纳米孔阵列结构

利用飞秒激光辐照研究了As2Se3表面激光诱导周期性表面结构（LIPSS）演化现象。在本实验中，周期性表面结构（LIPSS）通过控制脉冲数来控制，最终实现纳米孔阵列的精确制造。采用时域有限差分技术进行数值模拟，揭示其演化机理。我们发现，低空间频率LIPSS （LSFL）光栅的初始形成将改变电场的分布，并在随后的纳米孔阵列的产生中起着至关重要的作用。通过改变飞秒激光直写扫描速度，在As2Se3表面制备了1 ~ 5排纳米孔阵列。我们已经证明，纳米孔的整体和单个形态趋势证实了初始光栅对后续结构的重要性。最后，在As2Se3表面制备的大面积纳米孔阵列在结构色方面表现出良好的应用前景。

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来源期刊

Ceramics International 工程技术-材料科学：硅酸盐

CiteScore

9.40

自引率

15.40%

发文量

4558

审稿时长

25 days

期刊介绍： Ceramics International covers the science of advanced ceramic materials. The journal encourages contributions that demonstrate how an understanding of the basic chemical and physical phenomena may direct materials design and stimulate ideas for new or improved processing techniques, in order to obtain materials with desired structural features and properties. Ceramics International covers oxide and non-oxide ceramics, functional glasses, glass ceramics, amorphous inorganic non-metallic materials (and their combinations with metal and organic materials), in the form of particulates, dense or porous bodies, thin/thick films and laminated, graded and composite structures. Process related topics such as ceramic-ceramic joints or joining ceramics with dissimilar materials, as well as surface finishing and conditioning are also covered. Besides traditional processing techniques, manufacturing routes of interest include innovative procedures benefiting from externally applied stresses, electromagnetic fields and energetic beams, as well as top-down and self-assembly nanotechnology approaches. In addition, the journal welcomes submissions on bio-inspired and bio-enabled materials designs, experimentally validated multi scale modelling and simulation for materials design, and the use of the most advanced chemical and physical characterization techniques of structure, properties and behaviour. Technologically relevant low-dimensional systems are a particular focus of Ceramics International. These include 0, 1 and 2-D nanomaterials (also covering CNTs, graphene and related materials, and diamond-like carbons), their nanocomposites, as well as nano-hybrids and hierarchical multifunctional nanostructures that might integrate molecular, biological and electronic components.