Field-orientation-dependent magnetic phases in GdRu2Si2 probed with muon-spin spectroscopy

IF 3.7 2区 物理与天体物理 Q1 Physics and Astronomy Physical Review B Pub Date : 2025-02-27 DOI:10.1103/physrevb.111.054440
B. M. Huddart, A. Hernández-Melián, G. D. A. Wood, D. A. Mayoh, M. Gomilšek, Z. Guguchia, C. Wang, T. J. Hicken, S. J. Blundell, G. Balakrishnan, T. Lancaster
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Abstract

Centrosymmetric GdRu2Si2 exhibits a variety of multi-Q magnetic states as a function of temperature and applied magnetic field, including a square skyrmion-lattice phase. The material's behavior is strongly dependent on the direction of the applied field, with different phase diagrams resulting for fields applied parallel or perpendicular to the crystallographic c axis. Here, we present the results of muon-spin relaxation (μ+SR) measurements on single crystals of GdRu2Si2. Our analysis is based on the computation of muon stopping sites and consideration of quantum zero-point motion effects of muons, allowing direct comparison with the underlying spin textures in the material. The muon site is confirmed experimentally, using angle-dependent measurements of the muon Knight shift. Using transverse-field μ+SR with fields applied along either the [001] or [100] crystallographic directions, we distinguish between the magnetic phases in this system via their distinct muon response, providing additional evidence for the skyrmion and meron-lattice phases, while also suggesting the existence of RKKY-driven muon hyperfine coupling. Zero-field μ+SR provides clear evidence for a transition between two distinct magnetically ordered phases at 39 K. Published by the American Physical Society 2025
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用μ介子-自旋光谱探测 GdRu2Si2 中与磁场取向有关的磁相
中心对称的GdRu2Si2表现出多种多q磁态,这是温度和外加磁场的函数,包括一个方形的skyrron -lattice相。材料的行为强烈依赖于施加的场的方向,与平行或垂直于晶体学c轴的场产生不同的相图。本文报道了GdRu2Si2单晶的μ -自旋弛豫(μ+SR)测量结果。我们的分析是基于μ子停止点的计算和考虑μ子的量子零点运动效应,从而可以直接与材料中潜在的自旋织构进行比较。通过对介子奈特位移的角度相关测量,实验证实了介子位置。利用沿[001]或[100]晶体学方向施加的横向场μ+SR,我们通过不同的μ子响应来区分该系统中的磁相,为skyrmion和介子-晶格相提供了额外的证据,同时也表明存在rkky驱动的μ子超精细耦合。零场μ+SR在39k下提供了两个不同磁有序相之间转变的明确证据。2025年由美国物理学会出版
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来源期刊
Physical Review B
Physical Review B 物理-物理:凝聚态物理
CiteScore
6.70
自引率
32.40%
发文量
0
审稿时长
3.0 months
期刊介绍: Physical Review B (PRB) is the world’s largest dedicated physics journal, publishing approximately 100 new, high-quality papers each week. The most highly cited journal in condensed matter physics, PRB provides outstanding depth and breadth of coverage, combined with unrivaled context and background for ongoing research by scientists worldwide. PRB covers the full range of condensed matter, materials physics, and related subfields, including: -Structure and phase transitions -Ferroelectrics and multiferroics -Disordered systems and alloys -Magnetism -Superconductivity -Electronic structure, photonics, and metamaterials -Semiconductors and mesoscopic systems -Surfaces, nanoscience, and two-dimensional materials -Topological states of matter
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