High-resolution and high-performance full-color electroluminescent quantum dot light-emitting diodes

IF 17.1 1区 材料科学 Q1 CHEMISTRY, PHYSICAL Nano Energy Pub Date : 2025-02-27 DOI:10.1016/j.nanoen.2025.110817
Kaiyu Yang , Hongxi Zheng , Chao Zhong , Xingyun Huang , Qingkai Zhang , Kuibao Yu , Yuan Qie , Tao Chen , Hailong Hu , Fushan Li
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Abstract

The rapid development of near-eye display has put forward higher requirements for the resolution and image quality, while the performance of quantum dots (QDs) is virtually unlimited by pixel size, making them an ideal material for the next generation high-resolution display devices. However, there are still significant challenges in depositing multi-color pixels within the micron range and achieving high performance for the full-color quantum dot light emitting diodes (QLEDs). Herein, a combination of directional transfer printing and Langmuir-Blodgett (LB) technique was utilized to precisely transfer multi-color QDs arrays in the predetermined direction, and the full-color QDs arrays demonstrated fantastic morphology and uniform arrangement. As a result, the full-color QLEDs showed excellent performance with a resolution of 6350 pixels per inch (PPI), a luminance up to 62,947 cd/m2 and a peak external quantum efficiency (EQE) of 10.03 %. In addition, pixel spacing layers were introduced to further suppress electrical crosstalk and unwanted light emission, and the redundant part of emissive layers enabled QDs to be embedded into pixel spacing layers readily. The resulting full-color QLEDs with independent pixels exhibited a same high resolution of 6350 PPI, with a luminance of 35,427 cd/m2 and a peak EQE of 8.55 %. Our work represents the best performance of full-color QLEDs with both high efficiency and high resolution, which demonstrates great potential in the application of future near-eye displays.

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高分辨率和高性能的全彩电致发光量子点发光二极管
近眼显示的快速发展对分辨率和图像质量提出了更高的要求,而量子点的性能几乎不受像素大小的限制,使其成为下一代高分辨率显示设备的理想材料。然而,在微米范围内沉积多色像素并实现全彩量子点发光二极管(qled)的高性能方面仍然存在重大挑战。将定向转移印刷与Langmuir-Blodgett (LB)技术相结合,实现了多色量子点阵列在预定方向上的精确转移,得到了形貌奇特、排列均匀的全彩量子点阵列。结果表明,全彩qled的分辨率为6350像素/英寸(PPI),亮度高达62947 cd/m2,峰值外量子效率(EQE)为10.03%,表现出优异的性能。此外,引入像素间隔层进一步抑制电串扰和不必要的光发射,并且发射层的冗余部分使量子点易于嵌入到像素间隔层中。所得到的具有独立像素的全彩qled具有相同的高分辨率,为6350 PPI,亮度为35,427 cd/m2,峰值EQE为8.55%。我们的工作代表了全彩qled的最佳性能,具有高效率和高分辨率,在未来的近眼显示应用中具有很大的潜力。
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来源期刊
Nano Energy
Nano Energy CHEMISTRY, PHYSICAL-NANOSCIENCE & NANOTECHNOLOGY
CiteScore
30.30
自引率
7.40%
发文量
1207
审稿时长
23 days
期刊介绍: Nano Energy is a multidisciplinary, rapid-publication forum of original peer-reviewed contributions on the science and engineering of nanomaterials and nanodevices used in all forms of energy harvesting, conversion, storage, utilization and policy. Through its mixture of articles, reviews, communications, research news, and information on key developments, Nano Energy provides a comprehensive coverage of this exciting and dynamic field which joins nanoscience and nanotechnology with energy science. The journal is relevant to all those who are interested in nanomaterials solutions to the energy problem. Nano Energy publishes original experimental and theoretical research on all aspects of energy-related research which utilizes nanomaterials and nanotechnology. Manuscripts of four types are considered: review articles which inform readers of the latest research and advances in energy science; rapid communications which feature exciting research breakthroughs in the field; full-length articles which report comprehensive research developments; and news and opinions which comment on topical issues or express views on the developments in related fields.
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