Intelligent tetrahydrothiophene gas detection based on electrochemical sensor array.

IF 1.7 4区 工程技术 Q3 INSTRUMENTS & INSTRUMENTATION Review of Scientific Instruments Pub Date : 2025-03-01 DOI:10.1063/5.0226213
Guoqing Xiao, Xi Lai, Liang Ge, Yong He, Yi Teng
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Abstract

With extensive use of natural gas energy, various gas accidents occur frequently. Reasonable odorization of natural gas is an effective way to detect gas leakage in time and avoid gas explosions. Therefore, it is necessary to realize the identification and concentration detection of natural gas odorants to ensure early warning without degrading the gas quality. Given the cross-interference effect of electrochemical gas sensors and the poor accuracy of conventional analysis methods, this paper proposed a method based on principal component analysis and the K-nearest neighbor algorithm to realize gas recognition. In addition, the backpropagation-AdaBoost model combined with an electrochemical sensor array was employed to estimate the concentration of tetrahydrothiophene, an odorant in natural gas. The natural gas from the Chenghua district of Chengdu was used as the gas source to verify the reliability of the method. The experimental results show that the gas recognition rate reaches 90.17%, and the tetrahydrothiophene concentration detection average relative error reduced to 3.37%. The results demonstrate that the method can effectively improve the prediction accuracy and reduce the impact of cross-interference on the detection of tetrahydrothiophene. The method can provide technical support for natural gas odorant detection with great engineering significance for solving gas safety problems.

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基于电化学传感器阵列的智能四氢噻吩气体检测。
随着天然气能源的广泛使用,各种燃气事故时有发生。天然气合理加臭是及时发现燃气泄漏、避免燃气爆炸的有效途径。因此,有必要实现天然气气味剂的识别和浓度检测,以确保预警而不降低气体质量。针对电化学气体传感器的交叉干扰效应和传统分析方法准确度较差的问题,本文提出了一种基于主成分分析和k近邻算法的气体识别方法。此外,将反向传播- adaboost模型与电化学传感器阵列相结合,用于估计天然气中的气味剂四氢噻吩的浓度。以成都成化区天然气为气源,验证了方法的可靠性。实验结果表明,气体识别率达到90.17%,四氢噻吩浓度检测平均相对误差降至3.37%。结果表明,该方法能有效提高预测精度,减少交叉干扰对四氢噻吩检测的影响。该方法可为天然气异味检测提供技术支持,对解决天然气安全问题具有重要的工程意义。
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来源期刊
Review of Scientific Instruments
Review of Scientific Instruments 工程技术-物理:应用
CiteScore
3.00
自引率
12.50%
发文量
758
审稿时长
2.6 months
期刊介绍: Review of Scientific Instruments, is committed to the publication of advances in scientific instruments, apparatuses, and techniques. RSI seeks to meet the needs of engineers and scientists in physics, chemistry, and the life sciences.
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