Distinctness of Electroluminescence and Optical Gain in Laser Diodes with Wide Polar Quantum Wells

IF 6.7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Photonics Pub Date : 2025-03-06 DOI:10.1021/acsphotonics.4c02193
Mateusz Hajdel, Krzysztof Gołyga, Marcin Siekacz, Anna Feduniewicz-Żmuda, Czesław Skierbiszewski, Ulrich Theodor Schwarz, Grzegorz Muziol
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Abstract

Despite the ubiquity of semiconductor-based emitters in optoelectronic devices we use every day, obstacles still remain to unlock their full potential. One of these lies in long-wavelength GaN-based laser diodes (LDs). It is common knowledge that InGaN quantum wells (QWs) exhibit extremely large built-in polarization, which helps to obtain long-wavelength emission in light-emitting diodes, thanks to the large quantum-confined Stark effect. However, in this paper, it is shown that in order to achieve long-wavelength LDs, wide InGaN QWs might be preferential. The lasing wavelength for blue LDs can be even 20 nm longer in the case of wide QWs than in thin QWs for the same composition. The mechanisms behind these effects are explored by analyzing evolution of spontaneous emission, amplified spontaneous emission, optical gain, and quasi-Fermi level separation. It is shown that in wide QWs, the spontaneous emission originates from highly excited states. However, as the carrier density increases, quantum states with lower energy take over. Furthermore, population inversion, and thus lasing action, is obtained from the lowest excited states, resulting in long-wavelength lasing. The reported effects should also be observed in other polar materials with sufficiently thick QWs.

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宽极量子阱激光二极管的电致发光特性和光增益
尽管我们每天使用的光电器件中无处不在的半导体发射器,但释放其全部潜力的障碍仍然存在。其中之一是长波gan基激光二极管(ld)。众所周知,InGaN量子阱(qw)具有极大的内置极化,这有助于在发光二极管中获得长波发射,这得益于大量子限制的斯塔克效应。然而,本文表明,为了实现长波长的ld,宽InGaN qw可能是优先的。在相同成分的情况下,宽qw的蓝色ld的激光波长甚至可以比薄qw长20 nm。通过分析自发发射、放大自发发射、光学增益和准费米能级分离的演化,探讨了这些效应背后的机制。结果表明,在宽量子阱中,自发辐射来源于高激发态。然而,随着载流子密度的增加,具有较低能量的量子态取而代之。此外,从最低激发态获得了居群反转,从而产生了激光作用,从而产生了长波长激光。在其他具有足够厚量子阱的极性材料中也可以观察到报道的效应。
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来源期刊
ACS Photonics
ACS Photonics NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
11.90
自引率
5.70%
发文量
438
审稿时长
2.3 months
期刊介绍: Published as soon as accepted and summarized in monthly issues, ACS Photonics will publish Research Articles, Letters, Perspectives, and Reviews, to encompass the full scope of published research in this field.
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