Reservoir computing determined by nonlinear weight dynamics in Gd-doped CeO2/CeO2 bi-layered oxide memristors†

IF 5.1 2区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Journal of Materials Chemistry C Pub Date : 2025-02-20 DOI:10.1039/D4TC05041J
Sola Moon, Cheolhong Park, Yunyoung Jung, Kyeong-Sik Min, Hyunhyub Ko and Tae-Sik Yoon
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Abstract

Reservoir computing (RC) is an effective framework for processing spatiotemporal signals. Memristors are well-suited for physical reservoirs in hardware-based RC systems due to their nonlinear functions and memory characteristics. This study experimentally demonstrates an RC system using Pt/Gd-doped CeO2(GDC)/CeO2/Pt memristors. These devices exhibit time-dependent weight updates and decay characteristics, which are critical for extracting spatial and temporal features in RC applications. While previous research has explored implementing RC systems by exploiting the nonlinearity of memristors, there is a lack of systematic research on factors affecting the nonlinearity of memristors and analyzing the reservoir states. Using the time-dependent dynamics of Pt/GDC/CeO2/Pt memristors, this study extracts reservoir states under different pulse conditions and systematically analyzes the factors affecting the extraction of these states. Our findings demonstrate that nonlinearly mapped reservoir states can be linearly separated to achieve high-performance recognition and prediction in complex spatiotemporal tasks in RC systems. Finally, the RC performance of the memristor shows up to 90.5% accuracy in 4-bit pattern verification using the Modified National Institute of Standards and Technology (MNIST) database.

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基于非线性权动力学的掺钆CeO2/CeO2双层氧化物忆阻器储层计算[j]
储层计算(RC)是处理时空信号的有效框架。由于忆阻器的非线性功能和记忆特性,它非常适合于基于硬件的RC系统中的物理储存器。本研究通过实验证明了一种使用Pt/ gd掺杂的CeO2(GDC)/CeO2/Pt忆阻器的RC系统。这些器件表现出时间相关的权重更新和衰减特性,这对于提取RC应用中的空间和时间特征至关重要。虽然以往的研究已经探索了利用忆阻器的非线性来实现RC系统,但缺乏对影响忆阻器非线性的因素和储层状态分析的系统研究。利用Pt/GDC/CeO2/Pt忆阻器的时间依赖动力学,提取了不同脉冲条件下的储层状态,并系统分析了影响这些状态提取的因素。研究结果表明,非线性映射的储层状态可以线性分离,从而实现RC系统中复杂时空任务的高性能识别和预测。最后,使用修改后的美国国家标准与技术研究所(MNIST)数据库,该忆阻器的RC性能在4位模式验证中显示出高达90.5%的准确率。
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来源期刊
Journal of Materials Chemistry C
Journal of Materials Chemistry C MATERIALS SCIENCE, MULTIDISCIPLINARY-PHYSICS, APPLIED
CiteScore
10.80
自引率
6.20%
发文量
1468
期刊介绍: The Journal of Materials Chemistry is divided into three distinct sections, A, B, and C, each catering to specific applications of the materials under study: Journal of Materials Chemistry A focuses primarily on materials intended for applications in energy and sustainability. Journal of Materials Chemistry B specializes in materials designed for applications in biology and medicine. Journal of Materials Chemistry C is dedicated to materials suitable for applications in optical, magnetic, and electronic devices. Example topic areas within the scope of Journal of Materials Chemistry C are listed below. This list is neither exhaustive nor exclusive. Bioelectronics Conductors Detectors Dielectrics Displays Ferroelectrics Lasers LEDs Lighting Liquid crystals Memory Metamaterials Multiferroics Photonics Photovoltaics Semiconductors Sensors Single molecule conductors Spintronics Superconductors Thermoelectrics Topological insulators Transistors
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