Mechanosensing of Stimuli Changes with Magnetically Gated Adaptive Sensitivity.

IF 8.7 1区 化学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Materials Letters Pub Date : 2025-02-04 eCollection Date: 2025-03-03 DOI:10.1021/acsmaterialslett.4c02021
Xichen Hu, Xianhu Liu, Quan Xu, Olli Ikkala, Bo Peng
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Abstract

Inspired by biological sensors that characteristically adapt to varying stimulus ranges, efficiently detecting stimulus changes sooner than the absolute stimulus values, we propose a mechanosensing concept in which the resolution can be adapted by magnetic field (H) gating to detect small pressure-changes under a wide range of compressive stimuli. This is realized with resistive sensing by pillared H-driven assemblies of soft ferromagnetic electrically conducting particles between planar electrodes under a voltage bias. By modulation of H, the pillars respond with mechanically adaptable sensitivity. Higher H enhances current resolution, while it increases scatter among repeating measurements due to increased magnetic structural jamming between colloids in their assembly. To manage the trade-off between electrical resolution and scatter, machine learning is introduced for searching optimum H gatings, thus facilitating efficient pressure prediction. This approach suggests bioinspired pathways for developing adaptive stimulus-responsive mechanosensors, detecting subtle changes across varying stimuli levels with enhanced effectiveness through machine learning.

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机械感应刺激变化与磁控自适应灵敏度。
受生物传感器适应不同刺激范围的特点的启发,我们提出了一种机械传感概念,其中分辨率可以通过磁场(H)门控来适应,以检测大范围压缩刺激下的小压力变化。这是通过在电压偏置下的平面电极之间的软铁磁导电粒子柱状h驱动组件的电阻传感实现的。通过对H的调制,柱的响应具有机械适应性。较高的H提高了电流分辨率,但由于胶体之间的磁结构干扰增加,重复测量中的散射增加。为了管理电分辨率和散射之间的权衡,引入了机器学习来搜索最佳H门,从而促进有效的压力预测。这种方法提出了开发自适应刺激响应机械传感器的生物启发途径,通过机器学习提高效率,检测不同刺激水平的细微变化。
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来源期刊
ACS Materials Letters
ACS Materials Letters MATERIALS SCIENCE, MULTIDISCIPLINARY-
CiteScore
14.60
自引率
3.50%
发文量
261
期刊介绍: ACS Materials Letters is a journal that publishes high-quality and urgent papers at the forefront of fundamental and applied research in the field of materials science. It aims to bridge the gap between materials and other disciplines such as chemistry, engineering, and biology. The journal encourages multidisciplinary and innovative research that addresses global challenges. Papers submitted to ACS Materials Letters should clearly demonstrate the need for rapid disclosure of key results. The journal is interested in various areas including the design, synthesis, characterization, and evaluation of emerging materials, understanding the relationships between structure, property, and performance, as well as developing materials for applications in energy, environment, biomedical, electronics, and catalysis. The journal has a 2-year impact factor of 11.4 and is dedicated to publishing transformative materials research with fast processing times. The editors and staff of ACS Materials Letters actively participate in major scientific conferences and engage closely with readers and authors. The journal also maintains an active presence on social media to provide authors with greater visibility.
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