Modeling Acoustic Attenuation, Sound Velocity and Wave Propagation in Lithium-Ion Batteries via a Transfer Matrix

IF 5.1 4区 材料科学 Q2 ELECTROCHEMISTRY Batteries & Supercaps Pub Date : 2024-11-16 DOI:10.1002/batt.202400478
Simon Feiler, Dr. Lukas Gold, Dr. Sarah Hartmann, Dr. Guinevere A. Giffin
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Abstract

A simple 1D transfer matrix model of a battery is introduced and parametrized using harvested individual cell components at 0 % and 100 % SoC. This model allows for the calculation of group velocity and attenuation. The results of the model show good agreement with measured values, highlighting increased attenuation and group velocity at the resonances. This emphasizes the importance of selecting a suitable interrogation frequency for ultrasound investigations in lithium-ion batteries. The model accurately replicates the observed weakening of resonances with increasing SoC. Additionally, it provides the basis to fit US spectroscopy data in the future, enabling immediate determination of component thickness and the Young's modulus of individual components, along with aiding in the identification aging effects of the anode and cathode materials. The model can visualize wave propagation within the battery. At certain frequencies, standing waves form which could be used in high-intensity ultrasound applications targeted at individual cell components.

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来源期刊
CiteScore
8.60
自引率
5.30%
发文量
223
期刊介绍: Electrochemical energy storage devices play a transformative role in our societies. They have allowed the emergence of portable electronics devices, have triggered the resurgence of electric transportation and constitute key components in smart power grids. Batteries & Supercaps publishes international high-impact experimental and theoretical research on the fundamentals and applications of electrochemical energy storage. We support the scientific community to advance energy efficiency and sustainability.
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