Food Freshness Prediction Platform Utilizing Deep Learning-Based Multimodal Sensor Fusion of Volatile Organic Compounds and Moisture Distribution

IF 9.1 1区 化学 Q1 CHEMISTRY, ANALYTICAL ACS Sensors Pub Date : 2025-03-23 DOI:10.1021/acssensors.5c00254
Zepeng Gu, Qinyan Xu, Xiaoyao Wang, Xianfeng Lin, Nuo Duan, Zhouping Wang, Shijia Wu
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Abstract

Various sensing methods have been developed for food spoilage research, but in practical applications, the accuracy of these methods is frequently constrained by the limitation of single-source data and challenges in cross-validating multimodal data. To address these issues, a new method combining multidimensional sensing technology with deep learning-based dynamic fusion has been developed, which can precisely monitor the spoilage process of beef. This study designs a gas sensor based on surface-enhanced Raman scattering (SERS) to directly analyze volatile organic compounds (VOCs) adsorbed on MIL-101(Cr) with amine-specific adsorption for data collection while also evaluating the moisture distribution of beef through low-field nuclear magnetic resonance (LF-NMR), providing multidimensional recognition and readings. By introducing the self-attention mechanism and SENet scaling features into the multimodal deep learning model, the system is able to adaptively fuse and focus on the important features of the sensors. After training, the system can predict the storage time of beef under controlled storage conditions, with an R2 value greater than 0.98. Furthermore, it can provide accurate freshness assessments for beef samples under unknown storage conditions. Relative to single-modality methods, accuracy improves from 90 to over 97%. Overall, the newly developed dynamic fusion deep learning multimodal model effectively integrates multimodal information, enabling the fast and reliable monitoring of beef freshness.

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基于深度学习的挥发性有机化合物和水分分布融合多模态传感器的食品新鲜度预测平台
食品腐败研究已经发展了多种传感方法,但在实际应用中,这些方法的准确性经常受到单源数据的限制和多模态数据交叉验证的挑战。针对这些问题,本文提出了一种将多维感知技术与基于深度学习的动态融合相结合的牛肉腐败过程精确监测方法。本研究设计了一种基于表面增强拉曼散射(SERS)的气体传感器,通过胺特异性吸附直接分析MIL-101(Cr)吸附的挥发性有机化合物(VOCs)进行数据采集,同时通过低场核磁共振(LF-NMR)评估牛肉的水分分布,提供多维识别和读数。通过在多模态深度学习模型中引入自关注机制和SENet尺度特征,系统能够自适应地融合和关注传感器的重要特征。经过训练,该系统能够预测受控储存条件下牛肉的储存时间,R2值大于0.98。此外,它还可以对未知储存条件下的牛肉样品提供准确的新鲜度评估。相对于单模态方法,准确率从90%提高到97%以上。总体而言,新开发的动态融合深度学习多模态模型有效地集成了多模态信息,实现了对牛肉新鲜度的快速可靠监测。
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来源期刊
ACS Sensors
ACS Sensors Chemical Engineering-Bioengineering
CiteScore
14.50
自引率
3.40%
发文量
372
期刊介绍: ACS Sensors is a peer-reviewed research journal that focuses on the dissemination of new and original knowledge in the field of sensor science, particularly those that selectively sense chemical or biological species or processes. The journal covers a broad range of topics, including but not limited to biosensors, chemical sensors, gas sensors, intracellular sensors, single molecule sensors, cell chips, and microfluidic devices. It aims to publish articles that address conceptual advances in sensing technology applicable to various types of analytes or application papers that report on the use of existing sensing concepts in new ways or for new analytes.
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