Exploring the Transverse Thermoelectric Effect of 4H-SiC Single Crystal for the Applications of High-Energy Infrared Laser Detection

IF 6.7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Photonics Pub Date : 2025-03-24 DOI:10.1021/acsphotonics.4c02569
Yahui Huang, Jianyu Yang, Yong Wang, Bo Dai
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Abstract

Although the transverse thermoelectric (TTE) effect has been proposed for infrared (IR) laser detection, the development of cost-effective TTE materials for high-energy IR detection remains challenging. This work proposes a groundbreaking TTE material based on c-axis 4° tilted n-type 4H-SiC single crystals for IR laser detector applications. Pulsed lasers with wavelengths of 1080 nm and durations ranging from 5 to 40 ms were used as the irradiation sources. The voltages recorded on the 4H-SiC surface were demonstrated to originate from the TTE effect, driven by Seebeck coefficient anisotropy, as made evident by comparing signals from various electrode pairs. Additionally, the influence of the laser incidence angle on the peak voltage and decay time was investigated, which may enhance the theoretical understanding of the TTE effect. Furthermore, the response of the detectors at elevated temperatures, from room temperature (RT) to 400 °C, was evaluated. These results suggest that 4H-SiC single crystals are promising low-cost TTE materials for high-energy IR detection.

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探索4H-SiC单晶横向热电效应在高能红外激光探测中的应用
虽然已经提出了用于红外激光探测的横向热电(TTE)效应,但开发具有成本效益的用于高能红外探测的TTE材料仍然具有挑战性。这项工作提出了一种突破性的基于c轴4°倾斜n型4H-SiC单晶的红外激光探测器应用TTE材料。采用波长为1080 nm、持续时间为5 ~ 40 ms的脉冲激光作为辐照源。通过比较来自不同电极对的信号,证明了在4H-SiC表面记录的电压是由塞贝克系数各向异性驱动的TTE效应产生的。此外,还研究了激光入射角对峰值电压和衰减时间的影响,这有助于提高对TTE效应的理论认识。此外,还评估了探测器在室温(RT)至400℃高温下的响应。这些结果表明,4H-SiC单晶是一种很有前途的低成本高能红外探测TTE材料。
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来源期刊
ACS Photonics
ACS Photonics NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
11.90
自引率
5.70%
发文量
438
审稿时长
2.3 months
期刊介绍: Published as soon as accepted and summarized in monthly issues, ACS Photonics will publish Research Articles, Letters, Perspectives, and Reviews, to encompass the full scope of published research in this field.
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