Stabilization and emissions characteristics of CH4–H2 blends in a premixed jet stabilized combustor

IF 7.5 1区 工程技术 Q2 ENERGY & FUELS Fuel Pub Date : 2025-09-01 Epub Date: 2025-03-26 DOI:10.1016/j.fuel.2025.135059
Rishikesh Sampat, Niek Goselink, Kaushal Dave, Ferry Schrijer, Arvind Gangoli Rao
{"title":"Stabilization and emissions characteristics of CH4–H2 blends in a premixed jet stabilized combustor","authors":"Rishikesh Sampat,&nbsp;Niek Goselink,&nbsp;Kaushal Dave,&nbsp;Ferry Schrijer,&nbsp;Arvind Gangoli Rao","doi":"10.1016/j.fuel.2025.135059","DOIUrl":null,"url":null,"abstract":"<div><div>Low emissions and fuel flexibility are two important criteria required for gas turbine combustors to facilitate the energy transition to low-carbon fuels for propulsion and power applications. A jet-stabilized combustor, having both these characteristics, was operated with CH<sub>4</sub>–H<sub>2</sub> fuel mixtures with H<sub>2</sub> varying from 0 to 100 % and with varying equivalence ratios (<span><math><mi>ϕ</mi></math></span>). Comprehensive measurements were carried out of the velocity field using Particle Image Velocimetry (PIV), temperature and gas composition by traversing probes in the chamber, and flame topology using chemiluminescence imaging. The flow field in this combustor consists of a jet that undergoes recirculation, generating Central and Peripheral Recirculation Zones (CRZ and PRZ). The recirculation ratio in the PRZ is found to be twice that of the CRZ. Increasing H<sub>2</sub> % for the same <span><math><mi>ϕ</mi></math></span> leads to higher NO<sub><em>x</em></sub>. Ultra-low <span><math><mi>ϕ</mi></math></span> flames could be stabilized only at H<span><math><msub><mspace></mspace><mn>2</mn></msub><mo>≥</mo></math></span>50 %, which in turn leads to low NO<sub><em>x</em></sub> due to low adiabatic flame temperatures. The combination of temperature, gas composition (CO/NO), and chemiluminescence images is used to identify the extent and location of the reaction zone. Distributed reaction zones, stabilizing at around 30 % of the length of the chamber, are achieved at lean conditions, whereas an increase in H<sub>2</sub> % makes the reaction zone more compact and shifts upstream towards the burner head. Flame kernels are extracted from the instantaneous chemiluminescence images, and probability distribution functions for their aspect ratio and axial location are constructed. It is seen that reducing <span><math><mi>ϕ</mi></math></span> leads to low aspect ratio kernels that tend to occur further downstream, whereas increasing H<sub>2</sub> % leads to higher aspect ratio kernels, stabilizing upstream. These flame kernel statistics are also used to identify ignition modes (autoignition/flame propagation) for varying fuel H<sub>2</sub> % and inlet <span><math><mi>ϕ</mi></math></span> based on a hypothesis of flame stabilization mechanisms.</div></div>","PeriodicalId":325,"journal":{"name":"Fuel","volume":"395 ","pages":"Article 135059"},"PeriodicalIF":7.5000,"publicationDate":"2025-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Fuel","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0016236125007847","RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2025/3/26 0:00:00","PubModel":"Epub","JCR":"Q2","JCRName":"ENERGY & FUELS","Score":null,"Total":0}
引用次数: 0

Abstract

Low emissions and fuel flexibility are two important criteria required for gas turbine combustors to facilitate the energy transition to low-carbon fuels for propulsion and power applications. A jet-stabilized combustor, having both these characteristics, was operated with CH4–H2 fuel mixtures with H2 varying from 0 to 100 % and with varying equivalence ratios (ϕ). Comprehensive measurements were carried out of the velocity field using Particle Image Velocimetry (PIV), temperature and gas composition by traversing probes in the chamber, and flame topology using chemiluminescence imaging. The flow field in this combustor consists of a jet that undergoes recirculation, generating Central and Peripheral Recirculation Zones (CRZ and PRZ). The recirculation ratio in the PRZ is found to be twice that of the CRZ. Increasing H2 % for the same ϕ leads to higher NOx. Ultra-low ϕ flames could be stabilized only at H250 %, which in turn leads to low NOx due to low adiabatic flame temperatures. The combination of temperature, gas composition (CO/NO), and chemiluminescence images is used to identify the extent and location of the reaction zone. Distributed reaction zones, stabilizing at around 30 % of the length of the chamber, are achieved at lean conditions, whereas an increase in H2 % makes the reaction zone more compact and shifts upstream towards the burner head. Flame kernels are extracted from the instantaneous chemiluminescence images, and probability distribution functions for their aspect ratio and axial location are constructed. It is seen that reducing ϕ leads to low aspect ratio kernels that tend to occur further downstream, whereas increasing H2 % leads to higher aspect ratio kernels, stabilizing upstream. These flame kernel statistics are also used to identify ignition modes (autoignition/flame propagation) for varying fuel H2 % and inlet ϕ based on a hypothesis of flame stabilization mechanisms.
查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
CH4-H2混合物在预混合射流稳定燃烧室中的稳定性和排放特性
低排放和燃料灵活性是燃气轮机燃烧器促进推进和动力应用向低碳燃料过渡所需的两个重要标准。射流稳定燃烧室,具有这两个特点,与CH4-H2燃料混合物,H2变化从0到100 %和不同的等效比(ϕ)操作。利用粒子图像测速仪(PIV)对速度场进行了全面测量,利用室内穿越探针对温度和气体成分进行了全面测量,利用化学发光成像对火焰拓扑结构进行了全面测量。该燃烧室中的流场由经过再循环的射流组成,产生中央和外围再循环区(CRZ和PRZ)。PRZ的再循环率是CRZ的两倍。对于相同的φ,增加H2 %会导致更高的NOx。超低φ火焰只有在H2≥50 %时才能稳定,这反过来又导致低NOx,因为低绝热火焰温度。结合温度、气体组成(CO/NO)和化学发光图像来识别反应区的范围和位置。在稀薄条件下,分布的反应区稳定在燃烧室长度的30% %左右,而H2的增加 %使反应区更加紧凑,并向燃烧器头部上游移动。从瞬时化学发光图像中提取火焰核,构造其长宽比和轴向位置的概率分布函数。可以看出,减少ϕ导致低纵横比核,往往发生进一步下游,而增加H2 %导致更高的纵横比核,稳定上游。这些火焰核统计也用于识别点火模式(自燃/火焰传播)为不同的燃料H2 %和进口φ基于假设的火焰稳定机制。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 去求助
来源期刊
Fuel
Fuel 工程技术-工程:化工
CiteScore
12.80
自引率
20.30%
发文量
3506
审稿时长
64 days
期刊介绍: The exploration of energy sources remains a critical matter of study. For the past nine decades, fuel has consistently held the forefront in primary research efforts within the field of energy science. This area of investigation encompasses a wide range of subjects, with a particular emphasis on emerging concerns like environmental factors and pollution.
期刊最新文献
Progress in the study of soot formation in inverse diffusion flames Cobalt-driven phase transformation of tungsten carbide toward enhanced hydrogen evolution reaction Pyrolysis characteristics of bio-dried products from sewage sludge: biodegradation regulation and economic evaluation Mechanochemical grafting polymerization of fluorinated thioctic acid towards high-performance aluminum fuels The role of solvent in lignin hydrothermal liquefaction: its influence on conversion and phenolic monomer selectivity
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1