Investigating iodine-129 in coral cores along East Philippines as a tracer of the North Equatorial Current bifurcation and marker of the Anthropocene

IF 8.1 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Chemosphere Pub Date : 2025-03-28 DOI:10.1016/j.chemosphere.2025.144342
Angel T. Bautista VII , Sophia Jobien M. Limlingan , Jeff Darren G. Valdez , Mary Magareth T. Bauyon , Remjohn Aron H. Magtaas , Arvin M. Jagonoy , Joseph Michael D. Racho , Aldrin Jan E. Tabuso , John Kenneth C. Valerio , Araceli M. Monsada , Edwin E. Dumalagan Jr. , Keanu Jershon S. Sarmiento , Miwako Toya , Fernando P. Siringan , Hiroyuki Matsuzaki
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Abstract

Measuring 129I in natural archives is an excellent way of reconstructing the historical impacts of human nuclear activities (HNA) and tracing their transport through the environment. Currently, understanding of 129I transport from the North to the South Pacific Ocean is limited, given that most HNA were conducted in the northern hemisphere. Here, we show the 129I/127I time series of two coral cores, namely Calaguas and Cantilan, located along the north (Kuroshio Current) and south (Mindanao Current) bifurcations of the North Equatorial Current (NEC) – a crucial region that acts as a gateway from the North to the South Pacific Ocean. Measurement and mathematical modeling results show that HNA impacts are transported and divided almost equally between the north and south bifurcations of the NEC. Moreover, it takes around three years for the 129I signals from the Philippines to reach Australia. In recent times, when 129I in the Pacific Ocean has been more saturated, 129I transport from the North to the South Pacific Ocean appear to be affected by the variabilities associated with the El Niño Southern Oscillation and the Pacific Decadal Oscillation, as these influence the strengths and positions of the north and south bifurcations of the NEC. Lastly, our results affirm that 129I records are excellent candidates for marking the beginning of the Anthropocene.

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研究沿东菲律宾的珊瑚核中的碘-129作为北赤道洋流分岔的示踪剂和人类世的标志
在自然档案中测量129I是重建人类核活动(HNA)的历史影响并追踪其在环境中的运输的一种极好的方法。目前,由于大多数海航都是在北半球进行的,因此对从北太平洋到南太平洋的129I运输的了解有限。在这里,我们展示了两个珊瑚芯的129I/127I时间序列,即Calaguas和Cantilan,位于北赤道流(NEC)的北(黑潮)和南(棉兰老流)分叉处,这是一个从北到南太平洋的门户的关键区域。测量和数学建模结果表明,海航的影响在NEC的南北分支之间被传输和分配得几乎相等。此外,129I信号从菲律宾到达澳大利亚需要大约三年的时间。最近,当太平洋的129I饱和程度更高时,从北到南太平洋的129I输送似乎受到与El Niño南方涛动和太平洋年代际涛动相关的变率的影响,因为这些变率影响了NEC南北分支的强度和位置。最后,我们的结果证实129I记录是标志人类世开始的优秀候选人。
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来源期刊
Chemosphere
Chemosphere 环境科学-环境科学
CiteScore
15.80
自引率
8.00%
发文量
4975
审稿时长
3.4 months
期刊介绍: Chemosphere, being an international multidisciplinary journal, is dedicated to publishing original communications and review articles on chemicals in the environment. The scope covers a wide range of topics, including the identification, quantification, behavior, fate, toxicology, treatment, and remediation of chemicals in the bio-, hydro-, litho-, and atmosphere, ensuring the broad dissemination of research in this field.
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