Resource utilization of red mud with biochar to prepare high-efficiency denitration catalysts

IF 10 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Journal of Cleaner Production Pub Date : 2025-03-29 DOI:10.1016/j.jclepro.2025.145386
Bo Song , Zhenxing Shen , Zitong Wang , Guiling Zhou , Qin Peng , Hao Fan , Jia Liu
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Abstract

The preparation of denitration catalyst from red mud is one of the ways to realize high value resource utilization. Currently, the main challenges in preparing denitration catalysts from RM include high calcination temperatures with long durations, complex metal loading processes, and narrow high-efficiency temperature windows. In this study, the denitration catalyst R5B5-450 was prepared using RM and biochar through acidification, grinding, and calcination. This method can effectively improve the above problems. R5B5-450 achieved over 90 % NO conversion within the temperature range of 225–400 °C and demonstrated significant potential for application in treating real coal-fired flue gas. This work provides a reference for the effective utilization and reduction of RM while also contributing to reducing the production cost of denitration catalysts.

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赤泥与生物炭的资源化利用制备高效脱硝催化剂
以赤泥为原料制备脱硝催化剂是实现资源高价值利用的途径之一。目前,从RM制备脱硝催化剂的主要挑战是煅烧温度高、持续时间长、金属加载过程复杂、高效温度窗窄。本研究以RM和生物炭为原料,经酸化、研磨、煅烧制备脱硝催化剂R5B5-450。该方法可以有效地改善上述问题。R5B5-450在225-400°C的温度范围内实现了90%以上的NO转化率,在处理实际燃煤烟气方面显示出巨大的应用潜力。该工作为有效利用和减少RM提供了参考,同时也有助于降低脱硝催化剂的生产成本。
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来源期刊
Journal of Cleaner Production
Journal of Cleaner Production 环境科学-工程:环境
CiteScore
20.40
自引率
9.00%
发文量
4720
审稿时长
111 days
期刊介绍: The Journal of Cleaner Production is an international, transdisciplinary journal that addresses and discusses theoretical and practical Cleaner Production, Environmental, and Sustainability issues. It aims to help societies become more sustainable by focusing on the concept of 'Cleaner Production', which aims at preventing waste production and increasing efficiencies in energy, water, resources, and human capital use. The journal serves as a platform for corporations, governments, education institutions, regions, and societies to engage in discussions and research related to Cleaner Production, environmental, and sustainability practices.
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