Depolarization Field Controllable HfZrOx-Based Ferroelectric Capacitors for Physical Reservoir Computing System

IF 8.2 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Applied Materials & Interfaces Pub Date : 2025-03-31 DOI:10.1021/acsami.5c00213
Euncho Seo, Eunjin Lim, Jio Shin, Sungjun Kim
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Abstract

Reservoir computing as one of the artificial neural networks can process input signals in various ways, thereby showing strength in modeling data that changes over time. The reservoir is utilized in various fields because it is particularly energy efficient in learning and can exhibit powerful performance with relatively few trainings cost. This study emphasizes the significant advantages of the hafnium zirconium oxide (HZO) film in reservoir applications by controlling the depolarization field. The decay time of HZO-based ferroelectric memory devices is investigated, focusing on the impact of both ferroelectric layer thickness and interlayer (IL) thickness on physical reservoir computing system. Devices with HZO film thicknesses of 10, 15, and 20 nm were fabricated and characterized. Among these, the 15 nm HZO film demonstrated optimal thickness, exhibiting excellent ferroelectric properties, including enhanced orthorhombic phase (o-phase) formation and reliable short-term memory characteristics. When the optimized device for decay time is integrated into a reservoir computing system, it achieved a remarkable average accuracy of 93.42% in image recognition tasks, emphasizing its capability for high-precision computations.

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用于物理存储计算系统的去极化场可控 HfZrOx 基铁电容器
油藏计算作为人工神经网络的一种,可以以各种方式处理输入信号,从而在建模随时间变化的数据方面显示出强大的能力。由于该储层在学习上特别节能,并且可以以相对较少的培训成本表现出强大的性能,因此被广泛应用于各个领域。本研究强调了通过控制去极化场,氧化铪锆(HZO)薄膜在储层应用中的显著优势。研究了基于hzo的铁电存储器件的衰减时间,重点研究了铁电层厚度和层间厚度对物理储层计算系统的影响。制备了HZO薄膜厚度分别为10、15和20 nm的器件,并对其进行了表征。其中,15nm的HZO薄膜具有最佳厚度,表现出优异的铁电性能,包括增强的正交相(o相)形成和可靠的短期记忆特性。将优化后的衰减时间装置集成到油藏计算系统中,在图像识别任务中平均准确率达到了93.42%,突出了其高精度计算能力。
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来源期刊
ACS Applied Materials & Interfaces
ACS Applied Materials & Interfaces 工程技术-材料科学:综合
CiteScore
16.00
自引率
6.30%
发文量
4978
审稿时长
1.8 months
期刊介绍: ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.
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