Quenching Strong-Field Rescattering of Photoemitted Electrons from Metallic Nanotapers by Using Moderate Bias Fields

IF 6.7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Photonics Pub Date : 2025-03-31 DOI:10.1021/acsphotonics.5c00207
Germann Hergert, Rasmus Lampe, Christoph Lienau
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Abstract

The rescattering of photoemitted electrons with the ionized emitter is a central process in strong-field photoemission from atomic, molecular, and solid-state systems, resulting in characteristic rescattering plateaus in the photoelectron spectra. Recently, the appearance of such plateaus was also observed in the multiphoton photoemission regime from metallic nanostructures, raising questions about their effects on the dynamics of the photoemission process. Here, we analyze the effects of external static electric fields on electron rescattering from tungsten nanotapers illuminated by intense, few-cycle near-infrared laser pulses. In the strong-field regime, we observe distinct changes in the spectral shape of the plateau region. Time-dependent Schrödinger equation simulations of the photoemission dynamics show that this spectral reshaping is a signature of the suppression of recollisions at sufficiently high bias voltages. This suppression predicts the generation of low-energy electron pulses with few-femtosecond subcycle duration and emission characteristics that maintain this pulse duration over mesoscopic propagation distances in the 100 nm range. An experiment is proposed to directly probe the time structure of such subcycle electron pulses.

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用中等偏压场猝灭金属纳米锥光电子的强场重散射
在原子、分子和固态系统的强场光发射中,光电子与电离发射器的再散射是一个中心过程,导致光电子能谱中的特征再散射高原。最近,在金属纳米结构的多光子光发射体系中也观察到这种高原的出现,这就提出了它们对光发射过程动力学影响的问题。在此,我们分析了外部静电场对强、少周期近红外激光脉冲照射下钨纳米晶电子再散射的影响。在强场状态下,我们观察到高原地区的光谱形状有明显的变化。时间相关的Schrödinger光发射动力学方程模拟表明,这种光谱重塑是在足够高的偏置电压下抑制回忆的标志。这种抑制预测了低能量电子脉冲的产生,其亚周期持续时间为几飞秒,并且在100 nm范围内的介观传播距离内保持这种脉冲持续时间的发射特性。提出了一种直接探测亚周期电子脉冲时间结构的实验方法。
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来源期刊
ACS Photonics
ACS Photonics NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
11.90
自引率
5.70%
发文量
438
审稿时长
2.3 months
期刊介绍: Published as soon as accepted and summarized in monthly issues, ACS Photonics will publish Research Articles, Letters, Perspectives, and Reviews, to encompass the full scope of published research in this field.
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